Challenges and strategies of formulating low-temperature electrolytes in lithium-ion batteries

被引:38
|
作者
Qin, Mingsheng [1 ,2 ]
Zeng, Ziqi [1 ]
Cheng, Shijie [1 ]
Xie, Jia [1 ]
机构
[1] Huazhong Univ Sci & Technol, Sch Elect & Elect Engn, State Key Lab Adv Elect Engn & Technol, Wuhan 430074, Peoples R China
[2] Huazhong Univ Sci & Technol, Sch Mat Sci & Engn, State Key Lab Mat Proc & Die & Mould Technol, Wuhan, Peoples R China
来源
INTERDISCIPLINARY MATERIALS | 2023年 / 2卷 / 02期
基金
中国国家自然科学基金;
关键词
electrolyte; lithium-ion batteries; low temperatures; solvation structures; HIGH-ENERGY DENSITY; GRAPHITE ELECTRODE; ELECTROCHEMICAL PROPERTIES; NONAQUEOUS ELECTROLYTES; GRAPHITE/ELECTROLYTE INTERFACE; CARBONATE ELECTROLYTES; PROPYLENE CARBONATE; ESTER COSOLVENTS; HIGH-PERFORMANCE; CELLS;
D O I
10.1002/idm2.12077
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Lithium-ion batteries (LIBs) have monopolized energy storage markets in modern society. The reliable operation of LIBs at cold condition (<0 degrees C), nevertheless, is inevitably hampered by the sluggish kinetics and parasite reactions, which falls behind the increasing demands for portable electronics and electric vehicles. The electrolyte controls both Li+ transport and interfacial reaction, dictating the low-temperature performance substantially. Therefore, the rational formulation of electrolytes is significant for realizing superior low-temperature performance and broadening application niches of LIBs. Herein, we first discuss the kinetic limitations of low-temperature LIBs, highlighting the importance of electrolyte structure and interfacial chemistry. Then, the advancements for formulating subzero-temperature electrolyte are summarized with in-depth discussions about electrolyte formulation, solvation structure, interfacial chemistry, and low-temperature behaviors. Moreover, some opportunities for lithium metal batteries and the corresponding low-temperature electrolyte are covered. Finally, the major challenges and future perspectives are outlined for low-temperature LIBs.
引用
收藏
页码:308 / 336
页数:29
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