Research progress and outlook on photocatalytic conversion of methane to methanol

被引：8
作者：
Jia, Taikang [1 ,2 ]
Wang, Wenzhong [1 ,2 ,3 ]
机构：
[1] Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine M, 1295 Dingxi Rd, Shanghai 200050, Peoples R China
[2] Univ Chinese Acad Sci, Ctr Mat Sci & Optoelect Engn, 19 Yuquan Rd, Beijing 100049, Peoples R China
[3] Univ Chinese Acad Sci, Hangzhou Inst Adv Study, Sch Chem & Mat Sci, 1 Sub Lane Xiangshan, Hangzhou 310024, Peoples R China
来源：
CHEMCATCHEM | 2024年 / 16卷 / 09期
基金：
中国国家自然科学基金;
关键词：
methane; methanol; resource utilization; C-1; chemistry; reactive chlorine species; SINGLE-ATOM CATALYSTS; DECORATED ZINC-OXIDE; PARTIAL OXIDATION; SELECTIVE OXIDATION; ROOM-TEMPERATURE; AMBIENT CONDITIONS; OXYGEN; DIOXIDE; DESIGN; PHOTOOXIDATION;
D O I：
10.1002/cctc.202301279
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Methane, a main component of natural gas, shale gas, and combustible ice, is widely distributed in nature. The direct conversion and efficient utilization of methane have become crucial topics within the scientific community. However, two main challenges persist in this field: methane activation and overoxidation inhibition. Recently, research on this subject has reached its pinnacle stage. Herein, we present some works addressing these concerns, particularly employing photocatalytic approaches, and with a specific focus on strategies aimed at enhancing the selectivity towards methanol as the desired product. Finally, we discuss the existing challenges and propose potential solutions for advancing direct methane-to-methanol conversion technology.
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页数：14
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