Aerosol optical depth climatology from the high-resolution MAIAC product over Europe: differences between major European cities and their surrounding environments

被引:12
作者
Di Antonio, Ludovico [1 ]
Di Biagio, Claudia [2 ]
Foret, Gilles [1 ]
Formenti, Paola [2 ]
Siour, Guillaume [1 ]
Doussin, Jean-Francois [1 ]
Beekmann, Matthias [2 ]
机构
[1] Univ Paris Cite, Univ Paris Est Creteil, CNRS, LISA, F-94010 Creteil, France
[2] Univ Paris Est Creteil, Univ Paris Cite, CNRS, LISA, F-75013 Paris, France
关键词
WESTERN MEDITERRANEAN SEA; PARTICULATE MATTER PM2.5; PO VALLEY; SOURCE APPORTIONMENT; SURFACE REFLECTANCE; AIR-QUALITY; POLDER-3/PARASOL; 2005-2013; VERTICAL-DISTRIBUTION; ATMOSPHERIC AEROSOLS; ORGANIC AEROSOLS;
D O I
10.5194/acp-23-12455-2023
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The aerosol optical depth (AOD) is a derived measurement useful to investigate the aerosol load and its distribution at different spatio-temporal scales. In this work we use long-term (2000-2021) MAIAC (Multi-Angle Implementation of Atmospheric Correction) retrievals with 1 km resolution to investigate the climatological AOD variability and trends at different scales in Europe: a continental (30-60 circle N, 20 circle W-40 circle E), a regional (100 x 100 km2) and an urban-local scale (3 x 3 km2). The AOD climatology at the continental scale shows the highest values during summer (JJA) and the lowest during winter (DJF) seasons. Regional and urban-local scales are investigated for 21 cities in Europe, including capitals and large urban agglomerations. Analyses show AOD average (550 nm) values between 0.06 and 0.16 at the urban-local scale while also displaying a strong north-south gradient. This gradient corresponds to a similar one in the European background, with higher AOD being located over the Po Valley, the Mediterranean Basin and eastern Europe. Average enhancements of the local with respect to regional AOD of 57 %, 55 %, 39 % and 32 % are found for large metropolitan centers such as Barcelona, Lisbon, Paris and Athens, respectively, suggesting a non-negligible enhancement of the aerosol burden through local emissions. Negative average deviations are observed for other cities, such as Amsterdam (-17 %) and Brussels (-6 %), indicating higher regional background signal and suggesting a heterogeneous aerosol spatial distribution that conceals the urban-local signal. Finally, negative statistically significant AOD trends for the entire European continent are observed. A stronger decrease rate at the regional scale with respect to the local scale occurs for most of the cities under investigation.
引用
收藏
页码:12455 / 12475
页数:21
相关论文
共 158 条
[21]   Vertical distribution of aerosol optical properties in the Po Valley during the 2012 summer campaigns [J].
Bucci, Silvia ;
Cristofanelli, Paolo ;
Decesari, Stefano ;
Marinoni, Angela ;
Sandrini, Silvia ;
Groess, Johannes ;
Wiedensohler, Alfred ;
Di Marco, Chiara F. ;
Nemitz, Eiko ;
Cairo, Francesco ;
Di Liberto, Luca ;
Fierli, Federico .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2018, 18 (08) :5371-5389
[22]  
Cantrell C, 2022, B AM METEOROL SOC, V103, P599, DOI 10.1175/BAMS-D-21-0115.1
[23]   Transport of aerosols over the French Riviera - link between ground-based lidar and spaceborne observations [J].
Chazette, Patrick ;
Totems, Julien ;
Shang, Xiaoxia .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2019, 19 (06) :3885-3904
[24]   Validation of GRASP algorithm product from POLDER/PARASOL data and assessment of multi-angular polarimetry potential for aerosol monitoring [J].
Chen, Cheng ;
Dubovik, Oleg ;
Fuertes, David ;
Litvinov, Pavel ;
Lapyonok, Tatyana ;
Lopatin, Anton ;
Ducos, Fabrice ;
Derimian, Yevgeny ;
Herman, Maurice ;
Tanre, Didier ;
Remer, Lorraine A. ;
Lyapustin, Alexei ;
Sayer, Andrew M. ;
Levy, Robert C. ;
Hsu, N. Christina ;
Descloitres, Jacques ;
Li, Lei ;
Torres, Benjamin ;
Karol, Yana ;
Herrera, Milagros ;
Herreras, Marcos ;
Aspetsberger, Michael ;
Wanzenboeck, Moritz ;
Bindreiter, Lukas ;
Marth, Daniel ;
Hangler, Andreas ;
Federspiel, Christian .
EARTH SYSTEM SCIENCE DATA, 2020, 12 (04) :3573-3620
[25]   A surface reflectance correction model to improve the retrieval of MISR aerosol optical depth supported by MODIS data [J].
Chen, Lijuan ;
Wang, Ren ;
Wei, Geng ;
Han, Jiamei ;
Zha, Yong .
ADVANCES IN SPACE RESEARCH, 2021, 67 (02) :858-867
[26]   Aerosol optical properties derived from POLDER-3/PARASOL (2005-2013) over the Western Mediterranean Sea - Part 2: Spatial distribution and temporal variability [J].
Chiapello, Isabelle ;
Formenti, Paola ;
Kabuiku, Lydie Mbemba ;
Ducos, Fabrice ;
Tanre, Didier ;
Dulac, Francois .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2021, 21 (16) :12715-12737
[27]   Long-term variability of aerosol optical thickness in Eastern Europe over 2001-2014 according to the measurements at the Moscow MSU MO AERONET site with additional cloud and NO2 correction [J].
Chubarova, N. Y. ;
Poliukhov, A. A. ;
Gorlova, I. D. .
ATMOSPHERIC MEASUREMENT TECHNIQUES, 2016, 9 (02) :313-334
[28]   Global ammonia distribution derived from infrared satellite observations [J].
Clarisse, Lieven ;
Clerbaux, Cathy ;
Dentener, Frank ;
Hurtmans, Daniel ;
Coheur, Pierre-Francois .
NATURE GEOSCIENCE, 2009, 2 (07) :479-483
[29]   Source apportionment of air pollution in European urban areas: Lessons from the ClairCity project [J].
Coelho, S. ;
Ferreira, J. ;
Rodrigues, V. ;
Lopes, M. .
JOURNAL OF ENVIRONMENTAL MANAGEMENT, 2022, 320
[30]  
Colette A., 2016, EMEP: CCC-Report 1/2016