High-performance metal halide perovskite transistors

被引:83
作者
Liu, Ao [1 ]
Zhu, Huihui [1 ]
Bai, Sai [2 ]
Reo, Youjin [1 ]
Caironi, Mario [3 ]
Petrozza, Annamaria [3 ]
Dou, Letian [4 ]
Noh, Yong-Young [1 ]
机构
[1] Pohang Univ Sci & Technol, Dept Chem Engn, Pohang, South Korea
[2] Univ Elect Sci & Technol China, Inst Fundamental & Frontier Sci, Chengdu, Peoples R China
[3] Ist Italiano Tecnol, Ctr Nano Sci & Technol, Milan, Italy
[4] Purdue Univ, Davidson Sch Chem Engn, W Lafayette, IN USA
基金
新加坡国家研究基金会; 欧洲研究理事会;
关键词
FIELD-EFFECT TRANSISTORS; SOLAR-CELLS; LEAD-FREE; CHANNEL TRANSISTORS; CARRIER MOBILITIES; DEFECT TOLERANCE; RATIONAL DESIGN; THIN; SEMICONDUCTORS; TRANSPORT;
D O I
10.1038/s41928-023-01001-2
中图分类号
TM [电工技术]; TN [电子技术、通信技术];
学科分类号
0808 ; 0809 ;
摘要
Advances in metal halide perovskite semiconductors for optoelectronic devices have revived research interest in their applicability in transistors. Despite initial challenges affecting perovskite-based transistors in terms of reproducibility and ambient-temperature operation capability, notable performance improvements have been achieved through the fine-tuning of channel material compositions, thin-film processing and device engineering. However, critical insight into the electrical properties of the materials is lacking, and their potential for application in large-area and microscale electronics remains unclear. Here we explore the development of metal halide perovskite transistors and compare their characteristics with those of mainstream semiconductor technologies. We examine the electronic and structural properties of halide perovskites, and discuss key perovskite transistors developed so far, focusing on defect chemistry and corresponding electrical properties. We also consider the challenges that exist in developing next-generation electronics and circuits with perovskites, and highlight potential research areas for future development. This Perspective explores the development of metal halide perovskite transistors, examining the properties of halide perovskites and key perovskite transistors, and considering the challenges that exist in developing next-generation electronics and circuits using these devices.
引用
收藏
页码:559 / 571
页数:13
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