A stretchable, self-healing and semi-transparent nanogenerator for energy harvesting and sensing

被引:29
作者
Bagchi, Biswajoy [1 ,2 ]
Datta, Priyankan [1 ,2 ]
Fernandez, Carmen Salvadores [1 ,2 ]
Xu, Lulu [1 ,2 ]
Gupta, Priya [1 ,2 ]
Huang, Wei [2 ]
David, Anna L. [1 ,3 ,4 ]
Siassakos, Dimitrios [1 ,3 ,4 ]
Homer-Vanniasinkam, Shervanthi [1 ]
Tiwari, Manish K. [1 ,2 ]
机构
[1] Wellcome EPSRC Ctr Intervent & Surg Sci, UCL, London W1W 7TS, England
[2] Nanoengn Syst Lab, UCL Mech Engn, London WC1E 7JE, England
[3] Elizabeth Garrett Anderson Inst Womens Hlth, UCL, London WC1E 6AU, England
[4] NIHR Univ Coll London Hosp, BRC, 149 Tottenham Court Rd, London W1T 7DN, England
基金
英国工程与自然科学研究理事会; 欧洲研究理事会;
关键词
Hydrogel; Gold nanoparticles; Self-healing; Nanogenerator; Biocompatibility; GOLD NANOPARTICLES; TRIBOELECTRIC NANOGENERATOR; BORAX HYDROGELS; ACID HYDROGELS; TANNIC-ACID; SENSORS;
D O I
10.1016/j.nanoen.2022.108127
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Triboelectric nanogenerators (TENGs) with an ability to harvest mechanical energy from natural and human activities, have shown tremendous potential to realise self-powered electronic devices and sensors. However, in order for optimum utilization of biomechanical energy, TENGs need to have body or tissue mimicking properties without compromising performance. Herein, a new hydrogel based all-soft, self-healing and stretchable TENG is introduced which exhibits outstanding power generation capability surpassing existing competitors. This unique TENG is realized by using gold nanoparticles doped semi-transparent hydrogel as an electrode and Ecoflex as the triboelectric layer which integrates multifunctional properties including rapid self-healing in < 2 min, 900% stretchability, high conductivity, transparency and excellent biocompatibility with human dermal fibroblasts. The use of a gel electrode with both ionic and electronic conductivities underlines the importance of gold nanoparticles in enhancing the performance of soft TENGs. A 5 cm(2) device exhibits a prodigious power density of 1680 mWm(-2) with an energy conversion efficiency of approximate to 26%, which is the highest achieved so far in contem-porary hydrogel based TENGs. The moldable components allow easy fabrication of devices with tunable shapes and sizes that conforms to the human body and can power multiple electrical devices directly from body movements thus opening up possibilities for next generation self-powered wearable or implanted devices.
引用
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页数:12
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