Microscopic observation of two-level systems in a metallic glass model

被引:10
作者
Mocanu, Felix C. C. [1 ]
Berthier, Ludovic [2 ,3 ]
Ciarella, Simone [1 ]
Khomenko, Dmytro [4 ,5 ]
Reichman, David R. R. [4 ]
Scalliet, Camille [6 ]
Zamponi, Francesco [1 ]
机构
[1] Univ Paris, Univ PSL, Sorbonne Univ, Lab Phys Ecole Normale Super,ENS,CNRS, F-75005 Paris, France
[2] Univ Cambridge, Yusuf Hamied Dept Chem, Lensfield Rd, Cambridge CB2 1EW, England
[3] Univ Montpellier, CNRS, Lab Charles Coulomb L2C, F-34095 Montpellier, France
[4] Columbia Univ, Dept Chem, 3000 Broadway, New York, NY 10027 USA
[5] Sapienza Univ Roma, Dipartimento Fis, Ple A Moro 2, I-00185 Rome, Italy
[6] Univ Cambridge, Ctr Math Sci, DAMTP, Wilberforce Rd, Cambridge CB3 0WA, England
基金
欧洲研究理事会;
关键词
ELASTIC BAND METHOD; THERMAL-CONDUCTIVITY; TUNNELING SYSTEMS; STATES; UNIVERSAL; DYNAMICS; HEAT;
D O I
10.1063/5.0128820
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The low-temperature quasi-universal behavior of amorphous solids has been attributed to the existence of spatially localized tunneling defects found in the low-energy regions of the potential energy landscape. Computational models of glasses can be studied to elucidate the microscopic nature of these defects. Recent simulation work has demonstrated the means of generating stable glassy configurations for models that mimic metallic glasses using the swap Monte Carlo algorithm. Building on these studies, we present an extensive exploration of the glassy metabasins of the potential energy landscape of a variant of the most widely used model of metallic glasses. We carefully identify tunneling defects and reveal their depletion with increased glass stability. The density of tunneling defects near the experimental glass transition temperature appears to be in good agreement with experimental measurements. Published under an exclusive license by AIP Publishing.
引用
收藏
页数:16
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