A 3D-Printed Portable UV and Visible Photoreactor for Water Purification and Disinfection Experiments

被引:1
作者
Castro, Nelson [1 ,2 ,3 ]
Queiros, Joana M. [1 ,2 ,3 ,4 ]
Alves, Dinis C. [1 ,2 ,4 ]
Fernandes, Margarida M. Macedo [1 ,2 ,5 ,6 ,7 ]
Lanceros-Mendez, Senetxu [1 ,2 ,8 ,9 ]
Martins, Pedro M. [3 ,4 ]
机构
[1] Univ Minho, Phys Ctr Minho & Porto Univ CF UM UP, P-4710057 Braga, Portugal
[2] Univ Minho, LaPMET Lab Phys Mat & Emergent Technol, P-4710057 Braga, Portugal
[3] Int Iberian Nanotechnol Lab INL, P-4715330 Braga, Portugal
[4] Univ Minho, Ctr Mol & Environm Biol, P-4710057 Braga, Portugal
[5] Univ Minho, IB S Inst Res & Innovat Biosustainabil, P-4710057 Braga, Portugal
[6] Univ Minho, Ctr Microelectromechan Syst CMEMS, P-4800058 Guimaraes, Portugal
[7] Univ Minho, LABBELS Associate Lab, P-4800058 Guimaraes, Portugal
[8] UPV EHU Sci Pk, Basque Ctr Mat Applicat & Nanostruct, BCMaterials, Leioa 48940, Spain
[9] Basque Fdn Sci, IKERBASQUE, Bilbao 48009, Spain
关键词
portable photoreactor; photocatalysis; ciprofloxacin; water purification; 3D printing; WASTE-WATER; LIGHT; TIO2; PHOTOCATALYSIS; NANOPARTICLES; DEGRADATION; POLLUTANTS; REMOVAL;
D O I
10.3390/nano14060525
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Water scarcity and contamination are urgent issues to be addressed. In this context, different materials, techniques, and devices are being developed to mitigate contemporary and forthcoming water constraints. Photocatalysis-based approaches are suitable strategies to address water contamination by degrading contaminants and eliminating microbes. Photoreactors are usually designed to perform photocatalysis in a scalable and standardised way. Few or none have been developed to combine these characteristics with portability, flexibility, and cost effectiveness. This study reports on designing and producing a portable (490 g), low-cost, and multifunctional photoreactor that includes adjustable radiation intensity and two types of wavelengths (UV-A and visible), including combined agitation in a compact mechanism produced through 3D printing technology. The mechanical, electrical, and optical subsystems were designed and assembled into a robust device. It is shown that it is possible to apply radiations that can reach 65 mW/cm(2) and 110 mW/cm(2) using the installed visible and UV LEDs and apply mechanical agitation up to 200 rpm, all under a ventilated system. Regarding functionality, the photoreactor proof of concept indicated the ability to degrade similar to 80% and 30% ciprofloxacin under UV and visible irradiation of TiO2 and Ag/TiO2 nanoparticles. The device also showed the ability to eliminate E. coli bacteria, recurring to radiation set-ups and nanoparticles. Therefore, the originally designed and constructed photoreactor concept was characterised and functionally validated as an exciting and flexible device for lab-scaled or outdoor experiments, assuring standardised and comparable results.
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页数:14
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