Optical Properties of Conical Quantum Dot: Exciton-Related Raman Scattering, Interband Absorption and Photoluminescence

被引:6
作者
Gavalajyan, Sargis P. [1 ]
Mantashian, Grigor A. [1 ,2 ]
Kharatyan, Gor Ts. [1 ]
Sarkisyan, Hayk A. [1 ]
Mantashyan, Paytsar A. [1 ,2 ]
Baskoutas, Sotirios [3 ]
Hayrapetyan, David B. [1 ,2 ]
机构
[1] Russian Armenian Univ, Dept Gen Phys & Quantum Nanostruct, 123 Hovsep Emin Str, Yerevan 0051, Armenia
[2] NAS RA, Inst Chem Phys, 5-2 Paruyr Sevak St, Yerevan 0014, Armenia
[3] Univ Patras, Dept Mat Sci, Patras 26504, Greece
关键词
conical quantum dot; exciton; Raman scattering; interband absorption; photoluminescence; STRONG-CONFINEMENT APPROACH; SENSITIZED SOLAR-CELLS; REFRACTIVE-INDEX; DONOR-IMPURITY; SPECTROSCOPY; ELECTRON; STATES; SPECTRA; COEFFICIENT; EFFICIENCY;
D O I
10.3390/nano13081393
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
The current work used the effective mass approximation conjoined with the finite element method to study the exciton states in a conical GaAs quantum dot. In particular, the dependence of the exciton energy on the geometrical parameters of a conical quantum dot has been studied. Once the one-particle eigenvalue equations have been solved, both for electrons and holes, the available information on energies and wave functions is used as input to calculate exciton energy and the effective band gap of the system. The lifetime of an exciton in a conical quantum dot has been estimated and shown to be in the range of nanoseconds. In addition, exciton-related Raman scattering, interband light absorption and photoluminescence in conical GaAs quantum dots have been calculated. It has been shown that with a decrease in the size of the quantum dot, the absorption peak has a blue shift, which is more pronounced for quantum dots of smaller sizes. Furthermore, the interband optical absorption and photoluminescence spectra have been revealed for different sizes of GaAs quantum dot.
引用
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页数:13
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共 68 条
[41]   The Role of Ligands in Determining the Exciton Relaxation Dynamics in Semiconductor Quantum Dots [J].
Peterson, Mark D. ;
Cass, Laura C. ;
Harris, Rachel D. ;
Edme, Kedy ;
Sung, Kimberly ;
Weiss, Emily A. .
ANNUAL REVIEW OF PHYSICAL CHEMISTRY, VOL 65, 2014, 65 :317-339
[42]   PATH-INTEGRAL STUDY OF EXCITONS AND BIEXCITONS IN SEMICONDUCTOR QUANTUM DOTS [J].
POLLOCK, EL ;
KOCH, SW .
JOURNAL OF CHEMICAL PHYSICS, 1991, 94 (10) :6776-6781
[43]   HYDROGENIC IMPURITIES IN GAAS-(GA,AL)AS QUANTUM DOTS [J].
PORRASMONTENEGRO, N ;
PEREZMERCHANCANO, ST .
PHYSICAL REVIEW B, 1992, 46 (15) :9780-9783
[44]   OPTICAL-ABSORPTION IN SEMICONDUCTOR QUANTUM DOTS - A TIGHT-BINDING APPROACH [J].
RAMANIAH, LM ;
NAIR, SV .
PHYSICAL REVIEW B, 1993, 47 (12) :7132-7139
[45]   Intra-miniband absorption coefficient in GaAs/AlxGa1-xAs core/shell spherical quantum [J].
Rodriguez-Magdaleno, K. A. ;
Perez-Alvarez, R. ;
Martinez-Orozco, J. C. .
JOURNAL OF ALLOYS AND COMPOUNDS, 2018, 736 :211-215
[46]   A review on quantum dot sensitized solar cells: Past, present and future towards carrier multiplication with a possibility for higher efficiency [J].
Sahu, Anurag ;
Garg, Ashish ;
Dixit, Ambesh .
SOLAR ENERGY, 2020, 203 :210-239
[47]   Effects of external electric and magnetic fields on the linear and nonlinear optical properties of InAs cylindrical quantum dot with modified Po d schl-Teller and Morse confinement potentials [J].
Sargsian, T. A. ;
Mkrtchyan, M. A. ;
Sarkisyan, H. A. ;
Hayrapetyan, D. B. .
PHYSICA E-LOW-DIMENSIONAL SYSTEMS & NANOSTRUCTURES, 2021, 126
[48]   The finite element simulation for the shallow impurity in quantum dots [J].
Satori, H. ;
Sali, A. .
PHYSICA E-LOW-DIMENSIONAL SYSTEMS & NANOSTRUCTURES, 2013, 48 :171-175
[49]   Intersubband optical absorption in strained double barrier quantum well infrared photodetectors [J].
Shi, JJ ;
Goldys, EM .
IEEE TRANSACTIONS ON ELECTRON DEVICES, 1999, 46 (01) :83-88
[50]  
Shu Y., 2020, ANGEW CHEM, V132, P22496, DOI 10.1002/ange.202004857