Geochemical tracing of synoptic scale modern dust transport over the Northeast Arabian Sea during the southwest monsoon

被引:1
作者
Singh, Udisha [1 ,2 ]
Suresh, K. [3 ]
Prabhat, Priyesh [4 ]
Rahaman, Waliur [4 ]
Kumar, Ashwini [1 ,2 ]
机构
[1] CSIR Natl Inst Oceanog, Geol Oceanog Div, Goa 403004, India
[2] Acad Sci & Innovat Res AcSIR, Ghaziabad 201002, India
[3] Phys Res Lab, Geosci Div, Ahmadabad 380009, India
[4] Minist Earth Sci, Natl Ctr Polar & Ocean Res, Goa 403804, India
关键词
Mineral dust; Sr-Nd isotopes; Clay mineralogy; Trace elements; Arabian Sea; AFRICAN DUST; RED-SEA; PHYTOPLANKTON BLOOMS; PRIMARY PRODUCTIVITY; ATLANTIC-OCEAN; SEDIMENTS; DESERT; WIND; CLAY; ACCUMULATION;
D O I
10.1016/j.scitotenv.2023.164438
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
During the Southwest monsoon (SWM), aeolian dust is mainly supplied via wet deposition over the northeast Arabian Sea (NEAS). To understand their impact on the biogeochemistry of the Arabian Sea, it is important to identify their sources and characteristics. In this context, wet deposit particulate (WDP) samples were collected at a coastal station (Goa; 15.4 & DEG; N, 73.8 & DEG; E) in the NEAS during the SWM for three years. These samples were used to characterize and iden-tify mineral dust sources using mineralogical, elemental, and isotopic (Sr and Nd) signatures. The WDP samples were classified as Beginning of Monsoon (BM, June samples), Mid Monsoon (MM, July-August samples) and End of Mon-soon (EM, September samples). Clay mineralogical composition indicate high palygorskite content during BM, which subsequently found to decrease in MM, and almost negligible in EM. However, smectite is highest during MM, with moderate presence of palygorskite during this period. The considerable variation in the relative percentages of clay minerals suggests significant temporal variability in dust sources which is further corroborated by the radio -genic isotopic composition. A strong seasonality in the isotopic composition is observed with 87Sr/86Sr ratio being rel-atively less radiogenic during MM than the BM and highly radiogenic at the EM. Whereas & sigma;Nd values show an opposite trend to 87Sr/86Sr ratios throughout the monsoon, with more radiogenic & sigma;Nd in the MM, and less radiogenic at the EM. End member mixing plot indicate dominant contribution of dust from the Arabian Peninsula (ARB) and Northeast African (NEA) sources during BM and MM, while a shift towards the Thar desert and Southwest Asian (SWA) sources at the EM. Trace elements associated with different sources were quantified and suggest high Fe concentration is asso-ciated with NEA dust sources, despite ARB being major supplier of aeolian dust to the Arabian Sea.
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页数:15
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