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Physical Limit of Nonlinear Brownian Oscillators in Quantum Trap
被引:1
|作者:
Chen, Fangyuan
[1
]
Kou, Zepu
[1
]
Jiang, Zonghuiyi
[1
]
Guo, Wanlin
[1
]
Liu, Xiaofei
[1
]
机构:
[1] Nanjing Univ Aeronaut & Astronaut, State Key Lab Mech & Control Aerosp Struct, Key Lab Intelligent Nano Mat & Devices, Minist Educ, Nanjing 210016, Peoples R China
基金:
中国国家自然科学基金;
关键词:
VAN-DER-WAALS;
DYNAMICS;
SYSTEMS;
NANOSCALE;
FORCES;
MEMORY;
WATER;
D O I:
10.1021/acs.jpclett.3c03334
中图分类号:
O64 [物理化学(理论化学)、化学物理学];
学科分类号:
070304 ;
081704 ;
摘要:
Quantum trap, a quantum and thermal fluctuations-induced nonmonotonous potential, offers a chance to build up microscopic mechanical systems completely dominated by fluctuations. Here, we explore the physical limit of the effective damping ratio of the nonlinear Brownian oscillator in a quantum trap, set by the finite separation for avoiding molecular-scale effects on the trap potential and the surface confinement effect-induced diverging damping and random forces. The quasiharmonic approximations and Langevin dynamics simulations show that the lowest effective damping ratios of the suspended Au plate and Au sphere upon a Teflon coating of 10 nm can be similar to 210 and similar to 145, respectively, at room temperature. Perforation is proposed as an effective route to reduce the damping ratio (down to 6.4) by attenuating the surface confinement effect. An unexpected result due to the temperature dependences of dielectric function and viscosity of ethanol is a further reduced damping ratio at 400 K (1.3). The nonlinear Brownian oscillator in the quantum trap shows promise of probing near-boundary hydrodynamics at nanoscale.
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页码:1719 / 1725
页数:7
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