Experimental study of CO2 capture by nanoparticle-enhanced 2-amino-2-methyl-1-propanol aqueous solution

被引:2
作者
Zhang, Qiuli [1 ]
Ning, Zhongyi [1 ]
Li, Xuelian [1 ]
Ning, Xiaogang [2 ]
Wu, Fan [2 ]
Zhou, Jun [1 ]
机构
[1] Xian Univ Architecture & Technol, Sch Chem & Chem Engn, Xian 710055, Shaanxi, Peoples R China
[2] Shaanxi Beiyuan Chem Ind Grp Co Ltd, Jinjie Ind Pk, Shenmu 719319, Shaanxi, Peoples R China
关键词
CARBON-DIOXIDE CAPTURE; MASS-TRANSFER; GAS-ABSORPTION; PERFORMANCE ENHANCEMENT; REGENERATION; WATER; AMP; SOLUBILITY; NANOFLUIDS; PARTICLES;
D O I
10.1039/d3ra06767j
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
2-Amino-2-methyl-1-propanol (AMP) is often used as a moderator to enhance the CO2 capture capacity of absorbents due to its unique spatial site resistance structure, and relatively few studies have been conducted on the enhancement of AMP aqueous solutions by nanoparticles for CO2 capture. In order to investigate the effect of nanoparticles on the CO2 capture performance of AMP aqueous solution, different nanofluids were formulated in this paper using a two-step method, and a bubbling reactor and an oil bath were used as the experimental setup for absorption/desorption, and through comparative experiments, it was found that the type of nanoparticles, the solid content, and the different parameters have great influences on the CO2 absorption load and desorption rate. The experimental results show that the addition of TiO2 nanoparticles to the AMP base solution can accelerate the absorption-desorption mass transfer rate of CO2, and there exists an optimal solid content of 1 g L-1 (+/- 1.0%, +/- 2.5%); after multiple absorption-desorption experiments, good cycling performance can still be achieved. The experimental results of the nanofluid-promoted mass transfer mechanism are also illustrated and analyzed in this paper.
引用
收藏
页码:33644 / 33653
页数:10
相关论文
共 50 条
[21]   Determination of kinetics of CO2 absorption in solutions of 2-amino-2-methyl-1-propanol using a microfluidic technique [J].
Zheng, Chen ;
Zhao, Bochao ;
Wang, Kai ;
Luo, Guangsheng .
AICHE JOURNAL, 2015, 61 (12) :4358-4366
[22]   Inhibiting effect of 2-amino-2-methyl-1-propanol on gelatinous product formation in non-aqueous CO2 absorbents: Experimental study and molecular understanding [J].
Liu, Chao ;
Jing, Guohua ;
Zhu, Zongqiang ;
Fan, Yinming ;
Mo, Shengpeng ;
Zhang, Yanan ;
Wang, Dunqiu ;
Lv, Bihong ;
Fu, Mingming ;
Zhou, Xiaobin .
CHEMICAL ENGINEERING JOURNAL, 2024, 481
[23]   Experimental and theoretical investigation of solubility of carbon dioxide in concentrated aqueous solution of 2-amino-2-methyl-1-propanol and piperazine [J].
Dash, Sukanta Kumar ;
Samanta, Amar Nath ;
Bandyopadhyay, Syamalendu S. .
JOURNAL OF CHEMICAL THERMODYNAMICS, 2012, 51 :120-125
[24]   Comparison of rate-based and equilibrium-stage models of a packed column for post-combustion CO2 capture using 2-amino-2-methyl-1-propanol (AMP) solution [J].
Afkhamipour, Morteza ;
Mofarahi, Masoud .
INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL, 2013, 15 :186-199
[25]   Absorption and Desorption Heat of Carbon Dioxide Capture Based on 2-Amino-2-Methyl-1-Propanol [J].
Guo, Jia ;
Wang, Xin ;
Li, Yi ;
Li, Qingfang ;
Liu, Haili ;
Wang, Hui .
ENERGIES, 2025, 18 (05)
[26]   Solubility of CO2 in Piperazine (PZ) Activated Aqueous Solutions of 2-Amino-2-methyl-1-propanol (AMP) at Elevated Pressures [J].
Murshid, Ghulam ;
Shariff, Azmi Mohd. ;
Bustam, Mohammad Azmi ;
Ullah, Sami .
PROCESS AND ADVANCED MATERIALS ENGINEERING, 2014, 625 :233-236
[27]   Comparing CO2 removal characteristics of aqueous solutions of monoethanolamine, 2-amino-2-methyl-1-propanol, methyldiethanolamine and piperazine through absorption process [J].
Khan, Anoar Ali ;
Halder, G. N. ;
Saha, A. K. .
INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL, 2016, 50 :179-189
[28]   Kinetic effect and absorption performance of piperazine activator into aqueous solutions of 2-amino-2-methyl-1-propanol through post-combustion CO2 capture [J].
Khan, Anoar Ali ;
Halder, Gopinath ;
Saha, Asit Kumar .
KOREAN JOURNAL OF CHEMICAL ENGINEERING, 2019, 36 (07) :1090-1101
[29]   Comparative Study of CO2 Capture by Aqueous and Nonaqueous 2-Amino-2-methyl-1-propanol Based Absorbents Carried Out by 13C NMR and Enthalpy Analysis [J].
Barzagli, Francesco ;
Giorgi, Claudia ;
Mani, Fabrizio ;
Peruzzini, Maurizio .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2019, 58 (11) :4364-4373
[30]   Impact of speciation on CO2 capture performance using blended absorbent containing ammonia, triethanolamine and 2-amino-2-methyl-1-propanol [J].
Song, Hao-Yang ;
Jeon, Soo-Bin ;
Jang, Se-Yong ;
Lee, Sang-Sup ;
Kang, Seong-Kuy ;
Oh, Kwang-Joong .
KOREAN JOURNAL OF CHEMICAL ENGINEERING, 2014, 31 (07) :1237-1245