Fluorescence enhancement of PbS colloidal quantum dots from silicon metasurfaces sustaining bound states in the continuum

被引:8
|
作者
Liu, Li [3 ,4 ]
Wang, Ruxue [3 ,4 ]
Sun, Yuwei [1 ,2 ]
Jin, Yi [1 ,2 ]
Wu, Aimin [3 ,4 ]
机构
[1] Zhejiang Univ, Coll Opt Sci & Engn, Int Res Ctr Adv Photon, Ctr Opt & Electromagnet Res, Beijing 310058, Peoples R China
[2] Zhejiang Univ, Coll Opt Sci & Engn, Int Res Ctr Adv Photon, Hangzhou 310058, Peoples R China
[3] Chinese Acad Sci, Shanghai Inst Microsyst & Informat Technol, State Key Lab Funct Mat Informat, Shanghai 200050, Peoples R China
[4] Zhejiang Univ, Coll Opt Sci & Engn, Int Res Ctr Adv Photon, Hangzhou 310058, Peoples R China
基金
国家重点研发计划; 中国国家自然科学基金;
关键词
bound states in the continuum; fluorescence enhancement; metasurface; PbS quantum dot; NANOCRYSTALS; DRIVEN;
D O I
10.1515/nanoph-2023-0195
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
PbS colloidal quantum dots (CQDs) can be considered a promising lighting material, but their emission performance is mired by defect sites, strong photo-induced activity, and interaction with the environment. Here, we utilize periodic silicon metasurface sustaining a symmetry-protected bound state in the continuum to enhance the near-infrared emission of PbS CQDs at room temperature. In the experimental investigation, it is observed that the fluorescence of the coated PbS CQDs is enhanced by 10 times by the fabricated metasurface, and the emission peak has a quality factor up to 251 at wavelength 1408 nm. Meanwhile, the potential of this work in sensing is demonstrated by showing that the enhanced emission is disturbed by the introduction of sparse gold nanoparticles. In all, this work confirms that dielectric metasurfaces sustaining bound states in the continuum can be adopted to efficiently improve the emission performance of PbS CQDs which may find various practical applications including on-chip silicon-based optical sources and integrated sensors.
引用
收藏
页码:3159 / 3164
页数:6
相关论文
共 50 条
  • [41] Integration of Colloidal PbS/CdS Quantum Dots with Plasmonic Antennas and Superconducting Detectors on a Silicon Nitride Photonic Platform
    Elsinger, Lukas
    Gourgues, Ronan
    Zadeh, Iman E.
    Maes, Jorick
    Guardiani, Antonio
    Bulgarini, Gabriele
    Pereira, Silvania F.
    Dorenbos, Sander N.
    Zwiller, Val
    Hens, Zeger
    Van Thourhout, Dries
    NANO LETTERS, 2019, 19 (08) : 5452 - 5458
  • [42] Ultra-high-Q resonances in terahertz all-silicon metasurfaces based on bound states in the continuum
    Wang, Pengfei
    He, Fengyan
    Liu, Jianjun
    Shu, Fangzhou
    Fang, Bin
    Lang, Tingting
    Jing, Xufeng
    Hong, Zhi
    PHOTONICS RESEARCH, 2022, 10 (12) : 2743 - 2750
  • [43] Polarization-controlled third harmonic generation by quasi-bound states in the continuum in silicon nanopillar metasurfaces
    Xu, Haixia
    Du, Qian
    Xiao, Xuan
    Chen, Yihang
    APPLIED SURFACE SCIENCE, 2024, 672
  • [44] Ultra-high-Q resonances in terahertz all-silicon metasurfaces based on bound states in the continuum
    PENGFEI WANG
    FENGYAN HE
    JIANJUN LIU
    FANGZHOU SHU
    BIN FANG
    TINGTING LANG
    XUFENG JING
    ZHI HONG
    Photonics Research, 2022, (12) : 2743 - 2750
  • [45] High-Harmonic Generation from Resonant Dielectric Metasurfaces Empowered by Bound States in the Continuum
    Zograf, George
    Koshelev, Kirill
    Zalogina, Anastasiia
    Korolev, Viacheslav
    Hollinger, Richard
    Choi, Duk-Yong
    Zuerch, Michael
    Spielmann, Christian
    Luther-Davies, Barry
    Kartashov, Daniil
    Makarov, Sergey, V
    Kruk, Sergey S.
    Kivshar, Yuri
    ACS PHOTONICS, 2022, 9 (02) : 567 - 574
  • [46] Second harmonic generation from GaP metasurfaces using quasi-bound-states-in-the-continuum
    Anthur, A. P.
    Zhang, H.
    Dominguez, R. P.
    Kalashnikov, D.
    Ha, S. T.
    Mass, T. W. W.
    Kuznetsov, A.
    Krivitsky, L.
    2021 FIFTEENTH INTERNATIONAL CONGRESS ON ARTIFICIAL MATERIALS FOR NOVEL WAVE PHENOMENA (METAMATERIALS), 2021, : X317 - X318
  • [47] Carrier photoexcitation from levels in quantum dots to states of the continuum in lasing
    Asryan, LV
    Suris, RA
    SEMICONDUCTORS, 2001, 35 (03) : 343 - 346
  • [48] Carrier photoexcitation from levels in quantum dots to states of the continuum in lasing
    L. V. Asryan
    R. A. Suris
    Semiconductors, 2001, 35 : 343 - 346
  • [49] BOUND-STATES IN THE CONTINUUM FROM SUPERSYMMETRIC QUANTUM-MECHANICS
    PAPPADEMOS, J
    SUKHATME, U
    PAGNAMENTA, A
    PHYSICAL REVIEW A, 1993, 48 (05): : 3525 - 3531
  • [50] Active manipulation of accidental quasi bound states in the continuum in Sb2Se3-Silicon hybridized metasurfaces
    Ma, Tian
    Sang, Wei
    Tian, Jiangkun
    Yue, Shuai
    Ma, Li
    Wang, Doudou
    Li, Jun
    OPTICAL MATERIALS, 2024, 149