Gamma-Ray Spectroscopy for 237Np Using a Transition-Edge Sensor with a Thick-Trilayer Membrane

被引:0
作者
Kikuchi, T. [1 ]
Fujii, G. [1 ]
Hayakawa, R. [1 ,2 ]
Smith, R. [3 ]
Hirayama, F. [1 ]
Sato, Y. [1 ]
Kohjiro, S. [1 ]
Ukibe, M. [1 ]
Ohno, M. [3 ]
Sato, A. [1 ]
Yamamori, H. [1 ]
Hamaguchi, T. [4 ]
Yasumune, T. [4 ]
Ito, C. [4 ]
Takasaki, K. [4 ]
机构
[1] Natl Inst Adv Ind Sci & Technol, Tsukuba 3058568, Japan
[2] Tokyo Metropolitan Univ, Hachioji, Tokyo 1920397, Japan
[3] Univ Tokyo, Bunkyo Ku, Tokyo 1138656, Japan
[4] Japan Atom Energy Agcy, Oarai, Ibaraki 3111393, Japan
关键词
Gamma-ray spectroscopy; Neptunium; 237; Non-destructive analysis; Transuranic radionuclides; Transition edge sensor; Trilayer membrane;
D O I
10.1007/s10909-022-02867-w
中图分类号
O59 [应用物理学];
学科分类号
摘要
Gamma-ray transition edge sensors (TESs) are intensively studied not only to measure isotopic composition of nuclear materials but to monitor transuranic radionuclides inside the human body. We have recently proposed a thick-trilayer membrane as an alternative to silicon-nitride (SixNy) single-layer ones. It consists of silicon dioxide (SiO2), SixNy, and SiO2 layers. Their total thickness is 6.9 mu m and exhibits almost the same thermal conductance as conventional SixNy ones with 1-mu m thickness. The thick-trilayer membrane is expected to have better mechanical strength against implementing heavy-bulk absorbers. In this paper, the gamma-ray TES with the thick-trilayer membrane is used to carry out the spectroscopy for the nuclear radiation source. Neptunium-237 and its decay product Protactinium-233 emit 86.5 and 86.6-keV lines, respectively, and they are clearly resolved by four pixels with the full-width-half-maximum (FWHM) resolution of (43.7 +/- 0.9) eV. Furthermore, their intensity ratio agrees with the radioactive equilibrium between the two nuclides. Our experimental results predict that a vast array of pixel formats will reduce the statistical uncertainty in less measuring time.
引用
收藏
页码:207 / 213
页数:7
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