Recent progress of metal single-atom catalysts for energy applications

被引：94
作者：
Yang, Qingqing [1 ,2 ]
Jiang, Yafei [3 ,4 ]
Zhuo, Hongying [5 ,6 ]
Mitchell, Ellen M. [7 ]
Yu, Qi [1 ,2 ,3 ,4 ,5 ,6 ]
机构：
[1] Shaanxi Univ Technol, Sch Mat Sci & Engn, Hanzhong 723001, Peoples R China
[2] Shaanxi Univ Technol, Shaanxi Lab Catalysis, Hanzhong 723001, Peoples R China
[3] Southern Univ Sci & Technol, Dept Chem, Shenzhen 518055, Peoples R China
[4] Southern Univ Sci & Technol, Guangdong Prov Key Lab Catalysis, Shenzhen 518055, Peoples R China
[5] Tsinghua Univ, Dept Chem, Beijing, Peoples R China
[6] Tsinghua Univ, Key Lab Organ Optoelect & Mol Engn, Minist Educ, Beijing, Peoples R China
[7] Bridgewater Coll, Dept Chem, Bridgewater, VA 22812 USA
来源：
NANO ENERGY | 2023年 / 111卷
关键词：
Single-atom catalysts; Catalytic activity; Energy conversion; Environmental pollution remediation; N-DOPED CARBON; ONE-POT SYNTHESIS; EFFICIENT OXYGEN REDUCTION; ELECTROCATALYTIC HYDROGEN EVOLUTION; PHOTOCATALYTIC CO2 REDUCTION; NITROGEN REDUCTION; LAYER DEPOSITION; HIGHLY EFFICIENT; POROUS CARBON; COORDINATION ENVIRONMENT;
D O I：
10.1016/j.nanoen.2023.108404
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Single-atom catalysts (SACs) have received tremendous attention in heterogeneous catalysis because of their excellent catalytic performance and robust stability. Metal SACs have exhibited distinctive advantages in activity and selectivity and tunable interactions between the metal atoms and supports. In this review, we have sum-marized the preparation and performance of metal SACs that have energy-related applications including the oxygen reduction reaction, hydrogen evolution reaction, N2 reduction reaction, methane conversion, CO2 reduction reaction, CO oxidation reaction, biomass conversion, and environmental pollutant degradation. The current challenges of metal SAC reactions in industrial applications are analyzed. Finally, the development trends of SACs in energy applications are discussed.
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页数：31
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