Recent Trends in Plasmon-Assisted Photocatalytic CO2 Reduction

被引：30
作者：
Ciocarlan, Radu-George [1 ]
Blommaerts, Natan [1 ,2 ,3 ]
Lenaerts, Silvia [2 ,3 ]
Cool, Pegie [1 ]
Verbruggen, Sammy W. W. [2 ,3 ]
机构：
[1] Univ Antwerp, Dept Chem, Univplein 1, B-2610 Antwerp, Belgium
[2] Univ Antwerp, Dept Biosci Engn, Groenenborgerlaan 171, B-2020 Antwerp, Belgium
[3] Univ Antwerp, NANOlab Ctr Excellence, Groenenborgerlaan 171, B-2020 Antwerp, Belgium
来源：
CHEMSUSCHEM | 2023年 / 16卷 / 05期
关键词：
CO2; valorization; photocatalysis; plasmons; semiconductors; surface plasmon resonance; VISIBLE-LIGHT PHOTOCATALYST; CARBON NITRIDE NANOSHEETS; PHONON ENERGY RELAXATION; AMBIENT-PRESSURE; HIGHLY EFFICIENT; IN-SITU; ELECTRON THERMALIZATION; METAL NANOPARTICLES; GOLD NANOPARTICLES; HYDROCARBON FUELS;
D O I：
10.1002/cssc.202201647
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
Direct photocatalytic reduction of CO2 has become an highly active field of research. It is thus of utmost importance to maintain an overview of the various materials used to sustain this process, find common trends, and, in this way, eventually improve the current conversions and selectivities. In particular, CO2 photoreduction using plasmonic photocatalysts under solar light has gained tremendous attention, and a wide variety of materials has been developed to reduce CO2 towards more practical gases or liquid fuels (CH4, CO, CH3OH/CH3CH2OH) in this manner. This Review therefore aims at providing insights in current developments of photocatalysts consisting of only plasmonic nanoparticles and semiconductor materials. By classifying recent studies based on product selectivity, this Review aims to unravel common trends that can provide effective information on ways to improve the photoreduction yield or possible means to shift the selectivity towards desired products, thus generating new ideas for the way forward.
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页数：25
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