Study on the Fabrication of Ag Doped ZnO-TiO2 Hybrid Photocatalyst with Excellent Photocatalytic Activity and Its Photocatalytic Decarboxylation Performance

被引:2
作者
Mei, Xueqiao [1 ]
Li, Chunhu [1 ]
机构
[1] Ocean Univ China, Coll Chem & Chem Engn, Qingdao 266100, Peoples R China
关键词
Ag; ZnO-TiO2; photocatalysis; Rhodamine B; synergy; DEGRADATION; COMPOSITE; GRAPHENE; NANOPARTICLES; SYSTEM;
D O I
10.1007/s11802-023-5271-8
中图分类号
P7 [海洋学];
学科分类号
0707 ;
摘要
Photocatalyst Ag/ZnO-TiO2 was prepared by template method. The catalyst was characterized by XRD, SEM, and UV-vis DRS. Rhodamine B (RhB) and target pollutants were used to evaluate the photocatalytic performance of the catalyst under 40 W UV-lamp. The photocatalytic degradation mechanism of Rhodamine B was discussed through free radical quenching experiment. The experimental results show that hexagonal ZnO-TiO2 can be successfully prepared by template method, and nano Ag particles are evenly loaded on the catalyst. Under the reaction conditions of 1% catalyst input and 40 W UV-lamp, the catalytic degradation rate of RhB by Ag/ZnO-TiO2 was 98.28%. The photocatalytic degradation mechanism of Ag/ZnO-TiO2 was explored by free radical quenching experiment. The experimental results show that H+ and center dot OH play a major role in the photocatalytic degradation of RhB by Ag/ZnO-TiO2.
引用
收藏
页码:469 / 478
页数:10
相关论文
共 50 条
[11]   Photocatalytic activity of ZnO-TiO2 hierarchical nanostructure prepared by combined electrospinning and hydrothermal techniques [J].
Kanjwal, Muzafar A. ;
Barakat, Nasser A. M. ;
Sheikh, Faheem A. ;
Park, Soo Jin ;
Kim, Hak Yong .
MACROMOLECULAR RESEARCH, 2010, 18 (03) :233-240
[12]   UV-and Visible-Light Photocatalytic Activity of Simultaneously Deposited and Doped Ag/Ag(I)-TiO2 Photocatalyst [J].
Liu, Rui ;
Wang, Ping ;
Wang, Xuefei ;
Yu, Huogen ;
Yu, Jiaguo .
JOURNAL OF PHYSICAL CHEMISTRY C, 2012, 116 (33) :17721-17728
[13]   Simple fabrication of the Ag-Ag2O-TiO2 photocatalyst thin films on polyester fabrics by magnetron sputtering and its photocatalytic activity [J].
Yu, Hua-Liang ;
Wu, Qing-Xing ;
Wang, Jun ;
Liu, Li-Qin ;
Zheng, Biao ;
Zhang, Cheng ;
Shen, Yao-Guo ;
Huang, Chun-Lei ;
Zhou, Bi ;
Jia, Jun-Rong .
APPLIED SURFACE SCIENCE, 2020, 503
[14]   Effect of synthesis process steps on the structure and photocatalytic performance of ZnO-TiO2 composites [J].
Liu, Zhihui ;
Ren, Yuanwen ;
Yu, Yue ;
Shen, Kai ;
Hu, Kai ;
Zhou, Jiankang ;
Wu, Mengxuan ;
Liu, Shimin ;
Wang, Zixi .
CERAMICS INTERNATIONAL, 2024, 50 (02) :3168-3175
[15]   Preparation of Ag/TiO2 Nanotube and Its Photocatalytic Performance [J].
Wan Bin ;
Chen Mingbo ;
Zhou Xiying ;
Shen Jianian ;
Li Wenge .
RARE METAL MATERIALS AND ENGINEERING, 2009, 38 (11) :2012-2016
[16]   Photocatalytic activity of Ag/ZnO /AgO/TiO2 composite [J].
Bian, Haiqin ;
Zhang, Zhengmei ;
Xu, Xiaoli ;
Gao, Yang ;
Wang, Tao .
PHYSICA E-LOW-DIMENSIONAL SYSTEMS & NANOSTRUCTURES, 2020, 124 (124)
[17]   ZIF-8 derived Ag-doped ZnO photocatalyst with enhanced photocatalytic activity [J].
Yang, Xiaobing ;
Qiu, Liqing ;
Luo, Xuetao .
RSC ADVANCES, 2018, 8 (09) :4890-4894
[18]   Fabrication of a ternary plasmonic photocatalyst of Ag/AgVO3/RGO and its excellent visible-light photocatalytic activity [J].
Zhao, Wei ;
Li, Jinhai ;
Wei, Zhong Bo ;
Wang, Shaomang ;
He, Huan ;
Sun, Cheng ;
Yang, Shaogui .
APPLIED CATALYSIS B-ENVIRONMENTAL, 2015, 179 :9-20
[19]   Electrochemical behavior and photocatalytic performance of chlorpyrifos pesticide decontamination using Ni-doped ZnO-TiO2 nanocomposite [J].
Esfandian, Hossein ;
Cherati, Mostafa Rostamnejad ;
Khatirian, Mahdi .
INORGANIC CHEMISTRY COMMUNICATIONS, 2024, 159
[20]   Band gap coupling in photocatalytic activity in ZnO-TiO2 thin films [J].
Garcia-Ramirez, E. ;
Mondragon-Chaparro, M. ;
Zelaya-Angel, O. .
APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING, 2012, 108 (02) :291-297