Capturing transient core-to-core resonances in Kr in intense extreme-ultraviolet laser fields by electron-ion coincidence spectroscopy

被引：2

作者：

Fushitani, Mizuho ^{[1
,2
]}

Yamada, Makoto ^{[1
]}

Fujise, Hikaru ^{[1
]}

Owada, Shigeki ^{[2
,3
]}

Togashi, Tadashi ^{[2
,3
]}

Nakajima, Kyo ^{[2
,3
]}

Yabashi, Makina ^{[2
,3
]}

Matsuda, Akitaka ^{[1
,2
]}

Hikosaka, Yasumasa ^{[2
,4
]}

Hishikawa, Akiyoshi ^{[1
,2
,5
]}

机构：

[1] Nagoya Univ, Grad Sch Sci, Dept Chem, Nagoya, Aichi 4648602, Japan

[2] SPring 8 Ctr, RIKEN, Sayo, Hyogo 6795148, Japan

[3] Japan Synchrotron Radiat Res Inst, Sayo, Hyogo 6795198, Japan

[4] Univ Toyama, Inst Liberal Arts & Sci, Toyama 9300194, Japan

[5] Nagoya Univ, Res Ctr Mat Sci, Nagoya, Aichi 4648602, Japan

来源：

PHYSICAL REVIEW A | 2023年 / 107卷 / 02期

关键词：

PHOTOELECTRON-SPECTRA; CORRELATION SATELLITES; HIGH-RESOLUTION; PHOTOIONIZATION; XE;

D O I：

10.1103/PhysRevA.107.L021101

中图分类号：

O43 [光学];

学科分类号：

070207 ; 0803 ;

摘要：

Resonances between core-hole states have been long hypothesized to understand nonlinear responses of atoms and molecules exposed to intense x-ray free-electron laser (XFEL) pulses, but evaded clear identification in previous studies due to their transient nature. Here we report clear evidence of core-to-core resonances by state-of-the-art electron-ion coincidence spectroscopy on Kr atoms. The observed 3p-3d resonance manifested the significance in multiple ionization to highly charged states against the ultrafast core-hole decay. The present study, elucidating the role of the core-to-core resonance in electronic responses of matter to high-frequency laser fields, will advance our understanding of nonlinear spectroscopy and ultrafast imaging by ultrashort intense EUV and x-ray pulses.

引用

页数：7

共 49 条

[1] Multi-channel photodissociation and XUV-induced charge transfer dynamics in strong-field-ionized methyl iodide studied with time-resolved recoil-frame covariance imaging [J].

Allum, Felix ;

Anders, Nils ;

Brouard, Mark ;

Bucksbaum, Philip ;

Burt, Michael ;

Downes-Ward, Briony ;

Grundmann, Sven ;

Harries, James ;

Ishimura, Yudai ;

Iwayama, Hiroshi ;

Kaiser, Leon ;

Kukk, Edwin ;

Lee, Jason ;

Liu, Xiaojing ;

Minns, Russell S. ;

Nagaya, Kiyonobu ;

Niozu, Akinobu ;

Niskanen, Johannes ;

O'Neal, Jordan ;

Owada, Shigeki ;

Pickering, James ;

Rolles, Daniel ;

Rudenko, Artem ;

Saito, Shu ;

Ueda, Kiyoshi ;

Vallance, Claire ;

Werby, Nicholas ;

Woodhouse, Joanne ;

You, Daehyun ;

Ziaee, Farzaneh ;

Driver, Taran ;

Forbes, Ruaridh .

FARADAY DISCUSSIONS, 2021, 228 :571-596

[2] Absolute cross sections for the photoionization of 4d electrons in Xe+ and Xe2+ ions [J].

Andersen, P ;

Andersen, T ;

Folkmann, F ;

Ivanov, VK ;

Kjeldsen, H ;

West, JB .

JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 2001, 34 (10) :2009-2019

[3]

aps, US, DOI [10.1103/PhysRevA.107.L021101, DOI 10.1103/PHYSREVA.107.L021101]

[4] SUBSHELL PHOTOIONIZATION OF XE BETWEEN 40 AND 1000EV [J].

BECKER, U ;

SZOSTAK, D ;

KERKHOFF, HG ;

KUPSCH, M ;

LANGER, B ;

WEHLITZ, R ;

YAGISHITA, A ;

HAYAISHI, T .

PHYSICAL REVIEW A, 1989, 39 (08) :3902-3911

[5] Ultra-fast and ultra-intense x-ray sciences: first results from the Linac Coherent Light Source free-electron laser [J].

Bostedt, C. ;

Bozek, J. D. ;

Bucksbaum, P. H. ;

Coffee, R. N. ;

Hastings, J. B. ;

Huang, Z. ;

Lee, R. W. ;

Schorb, S. ;

Corlett, J. N. ;

Denes, P. ;

Emma, P. ;

Falcone, R. W. ;

Schoenlein, R. W. ;

Doumy, G. ;

Kanter, E. P. ;

Kraessig, B. ;

Southworth, S. ;

Young, L. ;

Fang, L. ;

Hoener, M. ;

Berrah, N. ;

Roedig, C. ;

DiMauro, L. F. .

JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 2013, 46 (16)

[6] ABSOLUTE OPTICAL OSCILLATOR-STRENGTHS FOR THE ELECTRONIC EXCITATION OF ATOMS AT HIGH-RESOLUTION .3. THE PHOTOABSORPTION OF ARGON, KRYPTON, AND XENON [J].

CHAN, WF ;

COOPER, G ;

GUO, X ;

BURTON, GR ;

BRION, CE .

PHYSICAL REVIEW A, 1992, 46 (01) :149-171

[7]

Condon E.U., 1953, THEORY ATOMIC SPECTR, V2nd

[8] AMO science at the FLASH and European XFEL free-electron laser facilities [J].

Feldhaus, J. ;

Krikunova, M. ;

Meyer, M. ;

Moeller, Th ;

Moshammer, R. ;

Rudenko, A. ;

Tschentscher, Th ;

Ullrich, J. .

JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 2013, 46 (16)

[9] Dynamics of Hollow Atom Formation in Intense X-Ray Pulses Probed by Partial Covariance Mapping [J].

Frasinski, L. J. ;

Zhaunerchyk, V. ;

Mucke, M. ;

Squibb, R. J. ;

Siano, M. ;

Eland, J. H. D. ;

Linusson, P. ;

v. d. Meulen, P. ;

Salen, P. ;

Thomas, R. D. ;

Larsson, M. ;

Foucar, L. ;

Ullrich, J. ;

Motomura, K. ;

Mondal, S. ;

Ueda, K. ;

Osipov, T. ;

Fang, L. ;

Murphy, B. F. ;

Berrah, N. ;

Bostedt, C. ;

Bozek, J. D. ;

Schorb, S. ;

Messerschmidt, M. ;

Glownia, J. M. ;

Cryan, J. P. ;

Coffee, R. N. ;

Takahashi, O. ;

Wada, S. ;

Piancastelli, M. N. ;

Richter, R. ;

Prince, K. C. ;

Feifel, R. .

PHYSICAL REVIEW LETTERS, 2013, 111 (07)

[10] X-ray induced ultrafast dynamics in atoms, molecules, and clusters: experimental studies at an X-ray free-electron laser facility SACLA and modelling [J].

Fukuzawa, Hironobu ;

Ueda, Kiyoshi .

ADVANCES IN PHYSICS-X, 2020, 5 (01)

← 1 2 3 4 5 →