Electrochromic-Induced Rechargeable Aqueous Batteries: An Integrated Multifunctional System for Cross-Domain Applications

被引:44
作者
Zhao, Qi [1 ,2 ]
Pan, Zhenghui [3 ]
Liu, Binbin [2 ]
Bao, Changyuan [2 ]
Liu, Ximeng [2 ]
Sun, Jianguo [2 ]
Xie, Shaorong [4 ]
Wang, Qing [2 ]
Wang, John [2 ,5 ,6 ]
Gao, Yanfeng [1 ,7 ]
机构
[1] Shanghai Univ, Dept Mat Sci & Engn, Shanghai 200444, Peoples R China
[2] Natl Univ Singapore, Dept Mat Sci & Engn, Singapore 117574, Singapore
[3] Tongji Univ, Dept Mat Sci & Engn, Shanghai 200092, Peoples R China
[4] Shanghai Univ, Dept Comp Engn & Sci, Shanghai 200444, Peoples R China
[5] Natl Univ Singapore Chongqing Res Inst, Chongqing 401120, Peoples R China
[6] ASTAR, Inst Mat Res & Engn, Singapore 138634, Singapore
[7] Chinese Acad Sci, Qinghai Inst Salt Lakes, Key Lab Comprehens & Highly Efficient Utilizat Sal, Xining 810008, Peoples R China
基金
新加坡国家研究基金会;
关键词
Electrochromic; Aqueous batteries; Multifunctional; Integration; ENERGY-STORAGE; PRUSSIAN BLUE; TUNGSTEN-OXIDE; SMART WINDOWS; DEVICE; FILMS; SUPERCAPACITOR; PROGRESS; WO3; ELECTROLYTES;
D O I
10.1007/s40820-023-01056-y
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Multifunctional electrochromic-induced rechargeable aqueous batteries (MERABs) integrate electrochromism and aqueous ion batteries into one platform, which is able to deliver the conversion and storage of photo- thermal-electrochemical sources. Aqueous ion batteries compensate for the drawbacks of slow kinetic reactions and unsatisfied storage capacities of electrochromic devices. On the other hand, electrochromic technology can enable dynamically regulation of solar light and heat radiation. However, MERABs still face several technical issues, including a trade-off between electrochromic and electrochemical performance, low conversion efficiency and poor service life. In this connection, novel device configuration and electrode materials, and an optimized compatibility need to be considered for multidisciplinary applications. In this review, the unique advantages, key challenges and advanced applications are elucidated in a timely and comprehensive manner. Firstly, the prerequisites for effective integration of the working mechanism and device configuration, as well as the choice of electrode materials are examined. Secondly, the latest advances in the applications of MERABs are discussed, including wearable, self- powered, integrated systems and multisystem conversion. Finally, perspectives on the current challenges and future development are outlined, highlighting the giant leap required from laboratory prototypes to large-scale production and eventual commercialization.
引用
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页数:31
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