Calorimetric evidence for two phase transitions in Ba1-xKxFe2As2 with fermion pairing and quadrupling states

被引:9
作者
Shipulin, Ilya [1 ,2 ]
Stegani, Nadia [3 ,4 ]
Maccari, Ilaria [5 ,6 ]
Kihou, Kunihiro [7 ]
Lee, Chul-Ho [7 ]
Hu, Quanxin [8 ]
Zheng, Yu [8 ]
Yang, Fazhi [8 ]
Li, Yongwei [8 ]
Yim, Chi-Ming [8 ,9 ]
Huehne, Ruben [1 ]
Klauss, Hans-Henning [2 ]
Putti, Marina [3 ,4 ]
Caglieris, Federico [3 ,4 ,10 ]
Babaev, Egor [5 ]
Grinenko, Vadim [8 ,9 ]
机构
[1] Leibniz IFW Dresden, Inst Met Mat, D-01069 Dresden, Germany
[2] Tech Univ Dresden, Inst Solid State & Mat Phys, D-01069 Dresden, Germany
[3] Univ Genoa, Via Dodecaneso 33, I-16146 Genoa, Italy
[4] Consiglio Nazl Ric CNR SPIN, Corso Perrone 24, I-16152 Genoa, Italy
[5] KTH Royal Inst Technol, Dept Phys, SE-10044 Stockholm, Sweden
[6] Paul Scherrer Inst, Lab Theoret & Computat Phys, CH-5232 Villigen, Switzerland
[7] Natl Inst Adv Ind Sci & Technol, Tsukuba, Ibaraki 3058568, Japan
[8] Shanghai Jiao Tong Univ, Tsung Dao Lee Inst, Shanghai 201210, Peoples R China
[9] Shanghai Jiao Tong Univ, Sch Phys & Astron, Shanghai, Peoples R China
[10] IFW Dresden, Leibniz Inst Solid State & Mat Res Dresden, D-01069 Dresden, Germany
基金
瑞典研究理事会;
关键词
PHASE-DIAGRAM; SUPERCONDUCTIVITY; VORTICES; FLUX; HEAT;
D O I
10.1038/s41467-023-42459-0
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Materials that break multiple symmetries allow the formation of four-fermion condensates above the superconducting critical temperature (T-c). Such states can be stabilized by phase fluctuations. Recently, a fermionic quadrupling condensate that breaks the Z(2) time-reversal symmetry was reported in Ba1-xKxFe2As2. A phase transition to the new state of matter should be accompanied by a specific heat anomaly at the critical temperature where Z(2) time-reversal symmetry is broken (T-c(Z2)>T-c). Here, we report on detecting two anomalies in the specific heat of Ba1-xKxFe2As2 at zero magnetic field. The anomaly at the higher temperature is accompanied by the appearance of a spontaneous Nernst effect, indicating the breakdown of Z(2) symmetry. The second anomaly at the lower temperature coincides with the transition to a zero-resistance state, indicating the onset of superconductivity. Our data provide the first example of the appearance of a specific heat anomaly above the superconducting phase transition associated with the broken time-reversal symmetry due to the formation of the novel fermion order.
引用
收藏
页数:9
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