Recent advances in quantum dot catalysts for hydrogen evolution: Synthesis, characterization, and photocatalytic application

被引:127
作者
Su, Haiwei [1 ]
Wang, Weikang [1 ]
Shi, Run [2 ]
Tang, Hua [1 ,3 ,4 ]
Sun, Lijuan [1 ]
Wang, Lele [1 ]
Liu, Qinqin [1 ,4 ]
Zhang, Tierui [2 ,5 ]
机构
[1] Jiangsu Univ, Sch Mat Sci & Engn, Zhenjiang, Jiangsu, Peoples R China
[2] Chinese Acad Sci, Optoelect Mat Tech Inst Phys & Chem, Key Lab Photochem Convers, Beijing, Peoples R China
[3] Qingdao Univ, Sch Environm Sci & Engn, Qingdao, Peoples R China
[4] Jiangsu Univ, Sch Mat Sci & Engn, Zhenjiang 212013, Jiangsu, Peoples R China
[5] Chinese Acad Sci, Optoelect Mat Tech Inst Phys & Chem, Key Lab Photochem Convers, Beijing 100190, Peoples R China
基金
中国国家自然科学基金;
关键词
characterization; functions of QDs; hydrogen evolution reaction; quantum dots; synthesis; GRAPHITIC CARBON NITRIDE; METAL-FREE PHOTOCATALYST; GREEN SYNTHESIS; HIGHLY EFFICIENT; UP-CONVERSION; HYDROTHERMAL SYNTHESIS; HIGH-PERFORMANCE; CARRIER SEPARATION; OPTICAL-PROPERTIES; CHARGE SEPARATION;
D O I
10.1002/cey2.280
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Photocatalytic water splitting is beneficial for the effective mitigation of global energy and environmental crises. Owing to multi-exciton generation, impressive light harvesting, and excellent photochemical properties, the quantum dot (QD)-based catalysts reveal a considerable potential in photocatalytic hydrogen (H-2) production compared with bulk competitors. In this review, we summarize the recent advances in QDs for photocatalytic H-2 production by enumerating different synthetic and characterization strategies for QDs. Various QDs-based photocatalysts are introduced and summarized in categories, and the role of different QDs in varied systems, as well as the mechanism and key factors that enhance the photocatalytic H-2 generation performance, is discussed. Finally, conclusions and future perspectives in the exploration of highly efficient QDs-based photocatalysts for innovative applications are highlighted.
引用
收藏
页数:37
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