Baseline Soil Dioxin Levels from Sites Where Municipal Solid Waste Incineration Construction Is Planned throughout China: Characteristics, Sources and Risk Assessment

被引:3
作者
Wan, Ruxing [1 ]
Wu, Jun [1 ]
Guo, Jing [2 ]
Qu, Jiabao [3 ]
Li, Ling [4 ]
Tang, Ling [1 ,5 ]
机构
[1] Beijing Univ Chem Technol, Sch Econ & Management, Beijing 100029, Peoples R China
[2] Beihang Univ, Sch Econ & Management, Beijing 100191, Peoples R China
[3] Minist Ecol & Environm, Appraisal Ctr Environm & Engn, Beijing 100012, Peoples R China
[4] Capital Univ Econ & Business, Int Sch Econ & Management, Beijing 100070, Peoples R China
[5] Univ Chinese Acad Sci, Sch Econ & Management, Beijing 100190, Peoples R China
基金
北京市自然科学基金; 中国国家自然科学基金;
关键词
dioxins; waste incineration; baseline levels; contaminant characteristics; health risk assessment; surface soil; DIBENZO-P-DIOXINS; HUMAN HEALTH-RISKS; POLYCYCLIC AROMATIC-HYDROCARBONS; PCDD/F CONCENTRATIONS; SPATIAL-DISTRIBUTION; POLYCHLORINATED-BIPHENYLS; ATMOSPHERIC DEPOSITION; AGRICULTURAL SOIL; RECYCLING SITES; SURFACE SOIL;
D O I
10.3390/su15129310
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The determination of baseline dioxins levels in soils is fundamental for the quantitative assessment of the net environmental and health impacts of municipal solid waste (MSW) incineration plants, which remains unexplored. Therefore, this study develops a Chinese baseline soil dioxins database (covering 918 soil samples from 292 pre-construction MSW incineration plants nationwide during 2016-2020) to thoroughly explore the baseline contamination characteristics and health risks of dioxins in soils. The empirical results show that (1) for concentration levels, the baseline international toxic equivalency (I-TEQ) concentrations vary from 0.0015 to 32 ng I-TEQ/kg, which are close to or even lower than those in most existing studies and show significant heterogeneity across provinces; (2) for dioxins homolog, highly chlorinated dioxins (i.e., PCDDs) are the dominant contributor to the total dioxins in soils (contributing 54.30% of the total I-TEQ concentrations), implying that dioxins in baseline soils often have an atmospheric fingerprint; and (3) for health risks, the carcinogenic risk and non-carcinogenic risk of dioxins in soils are mostly below acceptable levels, close to or even lower than the results of previous studies. Despite these results being considered as quite preliminary, they have certain implications for local authorities. Future studies can expand the size of the database and the generalizability of the results, and if necessary, establish a long-term dynamic monitoring of dioxins in soils for systematically evaluating the net impact of MSW incineration on environment and human health.
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页数:17
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