Towards ultralow platinum loading proton exchange membrane fuel cells

被引：104
作者：
Fan, Linhao [1 ]
Deng, Hao [2 ]
Zhang, Yingguang [3 ]
Du, Qing [1 ]
Leung, Dennis Y. C. [3 ]
Wang, Yun [4 ]
Jiao, Kui [1 ,5 ]
机构：
[1] Tianjin Univ, State Key Lab Engines, 135 Yaguan Rd, Tianjin 300350, Peoples R China
[2] Shanghai Hydrogen Prop Technol Co Ltd, 1788 Xiechun Rd, Shanghai 201804, Peoples R China
[3] Univ Hong Kong, Dept Mech Engn, Pokfulam Rd, Hong Kong, Peoples R China
[4] Univ Calif Irvine, Dept Mech & Aerosp Engn, Renewable Energy Resources Lab, Irvine, CA 92697 USA
[5] Tianjin Univ, Natl Ind Educ Platform Energy Storage, 135 Yaguan Rd, Tianjin 300350, Peoples R China
来源：
ENERGY & ENVIRONMENTAL SCIENCE | 2023年 / 16卷 / 04期
基金：
中国国家自然科学基金; 中国博士后科学基金;
关键词：
OXYGEN REDUCTION REACTION; CATHODE ELECTRODE; CATALYST LAYERS; REACTION-RATES; IONIC LIQUIDS; PERFORMANCE; IONOMER; NANOPARTICLES; DEGRADATION; FABRICATION;
D O I：
10.1039/d2ee03169h
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
With the upcoming worldwide commercialization of proton exchange membrane fuel cells (PEMFCs), the challenges regarding their cost, performance and durability urgently need to be overcome. Developing ultralow platinum (Pt) loading PEMFCs is a critical technical route to improve their cost competitiveness. This perspective provides in-depth discussion and insights on the motivation for an ultralow Pt loading of less than 0.05 grams per kilowatt, along with important technical development routes. The latest advancements for designing catalyst layers are presented regarding the critical mass transfer and degradation issues under low Pt loading. Moreover, approaches for accelerating catalyst layer development, including material development, structure design, and preparation technology, are proposed to meet the ultralow Pt loading target, which are expected to be implemented in next-generation catalyst layers for PEMFCs.
引用
收藏
页码：1466 / 1479
页数：15
相关论文
共 107 条
[21]   New roads and challenges for fuel cells in heavy-duty transportation [J].
Cullen, David A. ;
Neyerlin, K. C. ;
Ahluwalia, Rajesh K. ;
Mukundan, Rangachary ;
More, Karren L. ;
Borup, Rodney L. ;
Weber, Adam Z. ;
Myers, Deborah J. ;
Kusoglu, Ahmet .
NATURE ENERGY, 2021, 6 (05) :462-474
[22]   Application of Machine Learning in Optimizing Proton Exchange Membrane Fuel Cells: A Review [J].
Ding, Rui ;
Zhang, Shiqiao ;
Chen, Yawen ;
Rui, Zhiyan ;
Hua, Kang ;
Wu, Yongkang ;
Li, Xiaoke ;
Duan, Xiao ;
Wang, Xuebin ;
Li, Jia ;
Liu, Jianguo .
ENERGY AND AI, 2022, 9
[23]   Applying machine learning to boost the development of high-performance membrane electrode assembly for proton exchange membrane fuel cells [J].
Ding, Rui ;
Ding, Yiqin ;
Zhang, Hongyu ;
Wang, Ran ;
Xu, Zihan ;
Liu, Yide ;
Yin, Wenjuan ;
Wang, Jiankang ;
Li, Jia ;
Liu, Jianguo .
JOURNAL OF MATERIALS CHEMISTRY A, 2021, 9 (11) :6841-6850
[24]   Nano-scale control of the ionomer distribution by molecular masking of the Pt surface in PEMFCs [J].
Doo, Gisu ;
Yuk, Seongmin ;
Lee, Ji Hye ;
Choi, Sungyu ;
Lee, Dong-Hyun ;
Lee, Dong Wook ;
Hyun, Jonghyun ;
Kwon, Sung Hyun ;
Lee, Seung Geol ;
Kim, Hee-Tak .
JOURNAL OF MATERIALS CHEMISTRY A, 2020, 8 (26) :13004-13013
[25]   Pt/WO3/C nanocomposite with parallel WO3 nanorods as cathode catalyst for proton exchange membrane fuel cells [J].
Dou, Meiling ;
Hou, Ming ;
Li, Zhilin ;
Wang, Feng ;
Liang, Dong ;
Shao, Zhigang ;
Yi, Baolian .
JOURNAL OF ENERGY CHEMISTRY, 2015, 24 (01) :39-44
[26]   Low-PGM and PGM-Free Catalysts for Proton Exchange Membrane Fuel Cells: Stability Challenges and Material Solutions [J].
Du, Lei ;
Prabhakaran, Venkateshkumar ;
Xie, Xiaohong ;
Park, Sehkyu ;
Wang, Yong ;
Shao, Yuyan .
ADVANCED MATERIALS, 2021, 33 (06)
[27]   Recent Advances in Electrode Design Based on One-Dimensional Nanostructure Arrays for Proton Exchange Membrane Fuel Cell Applications [J].
Du, Shangfeng .
ENGINEERING, 2021, 7 (01) :33-49
[28]   Bridging the gap between highly active oxygen reduction reaction catalysts and effective catalyst layers for proton exchange membrane fuel cells [J].
Fan, Jiantao ;
Chen, Ming ;
Zhao, Zhiliang ;
Zhang, Zhen ;
Ye, Siyu ;
Xu, Shaoyi ;
Wang, Haijiang ;
Li, Hui .
NATURE ENERGY, 2021, 6 (05) :475-486
[29]   Enhancing oxygen transport in the ionomer film on platinum catalyst using ionic liquid additives [J].
Fan, Linhao ;
Wang, Yun ;
Jiao, Kui .
FUNDAMENTAL RESEARCH, 2022, 2 (02) :230-236
[30]   Oxygen Permeation Resistances and Routes in Nanoscale Ionomer Thin Film on Platinum Surface [J].
Fan, Linhao ;
Wang, Yun ;
Jiao, Kui .
JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2021, 168 (01)
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