Oxidation resistance and heat transfer simulation of MoSi2-based coatings on carbon fiber reinforced C-Al2O3 aerogel composite

被引:0
作者
Dai, Tao [1 ,2 ]
Wu, Zhanwu [3 ]
Wang, Zihan [1 ,2 ]
Cui, Sheng [1 ,2 ]
Wu, Xiaodong [1 ,2 ]
Zhu, Xiaofei [3 ]
机构
[1] Nanjing Tech Univ, Coll Mat Sci & Engn, State Key Lab Mat Oriented Chem Engn, Nanjing 210009, Peoples R China
[2] Nanjing Tech Univ, Suqian Adv Mat Ind Technol Innovat Ctr, Suqian 223800, Peoples R China
[3] Shanghai Space Prop Technol Res Inst, Huzhou 313000, Peoples R China
基金
中国国家自然科学基金;
关键词
Thermal protection; MoSi2-aluminoborosilicate coatings; Fiber-reinforced aerogel; Heat transfer simulation; THERMAL PROTECTION SYSTEM; SPECTRAL EMISSIVITY; BEHAVIOR;
D O I
10.1007/s10971-022-05746-8
中图分类号
TQ174 [陶瓷工业]; TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Fiber-reinforced aerogels with excellent properties such as low density and low thermal conductivity are potential thermal insulation materials. The slurry method and the embedding sintering method were used to fabricate MoSi2 aluminoborosilicate glass coatings on the surface of a carbon fiber-reinforced C-Al2O3 aerogel composite under a low-oxygen atmosphere. The microstructure and phase composition of the coatings with different MoSi2 contents before and after static oxidation were investigated. The resulting composite exhibited excellent radiating properties and outstanding oxidation resistance. The total emissivity of the as-prepared coatings was above 0.8185 in the wavelength range of 300-2500 nm. The sample with 40 wt% MoSi2 in the outer coating had superior thermal endurance with a weight loss of only 0.54% after isothermal oxidation at 1200 degrees C for 180 min. This can be attributed to the optimum viscosity of the binder, which would relieve thermal stress defects and block oxygen diffusion. To further evaluate the thermal protection performance of the coatings, the heat transfer characteristics were simulated using the Fluent software package. [GRAPHICS] .
引用
收藏
页码:393 / 405
页数:13
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