Visualizing temperature inhomogeneity using thermo-responsive smart materials

被引:8
|
作者
Wang, Panqin [1 ]
Du, Jiaren [1 ]
Wang, Tengyue [1 ]
Lyu, Shaoxing [1 ]
Van Deun, Rik [2 ]
Poelman, Dirk [3 ,4 ]
Lin, Hengwei [1 ]
机构
[1] Jiangnan Univ, Sch Chem & Mat Engn, Int Joint Res Ctr Photo Respons Mol & Mat, Wuxi 214122, Jiangsu, Peoples R China
[2] Univ Ghent, Dept Chem, Luminescent Lanthanide Lab L3, Krijgslaan 281-S3, B-9000 Ghent, Belgium
[3] Univ Ghent, Dept Solid State Sci, LumiLab, Krijgslaan 281-S1, B-9000 Ghent, Belgium
[4] Univ Ghent, Ctr Nano & Biophoton NB Photon, B-9000 Ghent, Belgium
基金
中国国家自然科学基金;
关键词
NANOPARTICLES;
D O I
10.1039/d3mh01198d
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Despite the substantial progress made, the responsiveness of thermo-responsive materials upon various thermal fields is still restricted to monochromatic visualization with single-wavelength light emission. This stems from a poor understanding of the photophysical processes within the materials and the unvarying optical performance of luminescent centers' response to various ambient temperatures. Conventional techniques to assess the inhomogeneities of thermal fields can be time-consuming, require specialized equipment and suffer from inaccuracy due to the inevitable interference from background signals, especially at high temperature. To this end, we overcome these limitations for the first time, to flexibly visualize temperature inhomogeneities by developing a thermochromic smart material, SrGa12-xAlxO19:Dy3+. Two distinct modes of thermochromic properties (steady-state temperature-dependent luminescence and thermally stimulated luminescence) are investigated. It is revealed that the abundant colors (from yellow, green to red) and amazing color-changing features are due to the superior optical integration of the host (SrGa12-xAlxO19) and dopant (Dy3+) emissions under specific thermal stimulations. We suggest that this thermo-responsive smart material can be used to realize highly efficient and simple visualization of invisible thermal distribution in industry and beyond. Thermo-responsive smart material with abundant colors and amazing color-changing luminescence feature can achieve highly efficient and simple visualization of invisible thermal distribution in industry and beyond.
引用
收藏
页码:5684 / 5693
页数:10
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