Influence of Rock Structure on Migration of Radioactive Colloids from an Underground Repository of High-Level Radioactive Waste

被引:2
作者
Malkovsky, Victor I. [1 ]
Petrov, Vladislav A. [1 ]
Yudintsev, Sergey V. [1 ]
Ojovan, Michael I. [1 ]
Poluektov, Valeri V. [1 ]
机构
[1] Russian Acad Sci, Inst Geol Ore Deposits Petrog Mineral & Geochem, Staromonetny Lane 35, Moscow 119017, Russia
关键词
radioactive waste; underground repository; radiocolloid; migration; ground water; fractures; mechanical retention; NUCLEAR-WASTE; TRANSURANIC RADIONUCLIDES; WATER; PLUTONIUM; DISPOSAL; AMERICIUM; PARTICLES; TRANSPORT; STABILITY; MATRIX;
D O I
10.3390/su15010882
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Studies of leaching of vitrified simulated high-level radioactive waste (HLW) evidence that most of actinides or their simulators enter leaching water in a colloidal form. In this paper, we consider a mechanism of colloid-facilitated migration of radionuclides from an underground repository of HLW located at a depth of a few hundreds of meters in fractured crystalline rocks. The comparison between data of field and laboratory measurements showed that the bulk permeability of the rock massif in field tests is much greater than the permeability of rock samples in laboratory experiments due to an influence of a network of fractures in the rock massif. Our theoretical analysis presents evidence that this difference can take place even in a case when the network is not continuous, and the fractures are isolated with each other through a porous low-permeable matrix of the rock. Results of modelling revealed a possibility of mechanical retention of radionuclide-bearing colloid particles in the frame of rock during their underground migration.
引用
收藏
页数:10
相关论文
共 41 条
[1]  
Barenblatt G.E., 1960, J APPL MATH USSR, V24, P12861303, DOI DOI 10.1016/0021-8928(60)90107-6
[2]  
Bear J., 1993, Flow and Contaminant Transport in Fractured Rock, DOI [10.1016/B978-0-12-083980-3.50005-X, DOI 10.1016/B978-0-12-083980-3.50005-X]
[3]   Flow in Fractured Porous Media: A Review of Conceptual Models and Discretization Approaches [J].
Berre, Inga ;
Doster, Florian ;
Keilegavlen, Eirik .
TRANSPORT IN POROUS MEDIA, 2019, 130 (01) :215-236
[4]  
Bredehoeft J.D., 1990, ROLE FLUIDS CRUSTAL, P27
[5]   Microanalysis of colloids and suspended particles from nuclear waste glass alteration [J].
Buck, EC ;
Bates, JK .
APPLIED GEOCHEMISTRY, 1999, 14 (05) :635-653
[6]  
De Marsily G., 1986, Quantitative Hydrology, P440
[7]   Colloid generation during water flow transients [J].
Degueldre, Claude ;
Benedicto, Ana .
APPLIED GEOCHEMISTRY, 2012, 27 (06) :1220-1225
[8]   Geological Disposal of Nuclear Waste: a Primer [J].
Ewing, Rodney C. ;
Whittleston, Robert A. ;
Yardley, Bruce W. D. .
ELEMENTS, 2016, 12 (04) :233-237
[9]   Geochemistry - Colloidal culprits in contamination [J].
Honeyman, BD .
NATURE, 1999, 397 (6714) :23-24
[10]   Effects of water redox conditions and presence of magnetite on leaching of Pu and Np from HLW glass [J].
Inagaki, Y ;
Sakata, H ;
Furuya, H ;
Idemitsu, K ;
Arima, T ;
Banba, T ;
Maeda, T ;
Matsumoto, S ;
Tamura, Y ;
Kikkawa, S .
SCIENTIFIC BASIS FOR NUCLEAR WASTE MANAGEMENT XXI, 1998, 506 :177-184