Dielectric prοperties and cοmplex impedance οf the 0.69PbMg1/3Nb2/3Ο3-0.31PbTiΟ3 relaxοr ceramic

被引:0
作者
Hnawi, Salma Kaotar [1 ,2 ]
Lifi, Houda [3 ,4 ]
Lifi, Mohamed [5 ]
Khrissi, Salam [3 ,6 ]
Benkhouja, Khalil [3 ]
Ali, Mustapha Ait [2 ]
机构
[1] Cadi Ayyad Univ, Fac Sci Semlalia, Lab Mat Energy & Environm Lab LaMEE, Marrakech, Morocco
[2] Cadi Ayyad Univ, Fac Sci Semlalia, Coordinat Chem & Catalysis Unit, Mol Chem Lab, Marrakech, Morocco
[3] Cadi Ayyad Univ, Natl Sch Appl Sci, Lab Mat Proc Environm & Qual, Safi, Morocco
[4] Chouaib Doukkali Univ, Fac Sci, Lab Innovat Sci Technol & Modeling LISTM, El Jadida, Morocco
[5] Univ Valladolid, Grp Energia Econ & Dinam Sistemas GEEDS, Valladolid, Spain
[6] Moulay Ismail Univ, Fac Sci, Lab Spectrometry Mat & Archaeomat LASMAR, Meknes, Morocco
关键词
Impedence spectroscopic; Electric permittivity; 0; 69PMN-0; 31PT; Complex modulus; SPECTROSCOPY; BEHAVIOR;
D O I
10.1080/01411594.2023.2227315
中图分类号
O7 [晶体学];
学科分类号
0702 ; 070205 ; 0703 ; 080501 ;
摘要
Impedance spectroscopy assessed dielectric properties of PMN at a single PT concentration. Real and imaginary impedance of (1-x) PMN-xPT materials were analyzed using this technique. Through electrical impedance spectroscopy, the loss tangent factor and electric modulus were determined, leveraging research on semiconductor conduction. The study also presented the synthesis and characterization of solid ceramic lead magnesium nibate-lead titanate (1-x) PbMg1/3Nb2/3-xPbTi3, representing a significant advancement in impedance spectroscopy research. The dielectric behavior was examined by studying the polarization evolution in response to the applied field, aiming to replicate the magnetic phase boundary configuration found in typical ferroelectric behavior. Temperature had a notable impact on the hysteresis loop, with increasing temperature and decreasing applied field resulting in decreased leftover polarization and increased coercive field. The impedance and complex modulus graphs exhibited distinct semicircle patterns attributed to higher grain boundary resistance and capacitance compared to (1-x) PMN-xPT. The Nyquist plot highlighted bulk effects.
引用
收藏
页码:366 / 374
页数:9
相关论文
共 33 条
[11]  
El Bouziani N., 2018, SURFACE ACOUSTIC WAV
[12]   Impedance spectroscopy of the relaxor behaviour of PMN and La-doped PMN-PT compositions [J].
Gupta, SM ;
Prasad, NV ;
Wadhawan, VK .
FERROELECTRICS, 2005, 326 :43-47
[13]   UNIVERSAL DIELECTRIC RESPONSE [J].
JONSCHER, AK .
NATURE, 1977, 267 (5613) :673-679
[14]   Study of marbles from Middle Atlas (Morocco): elemental, mineralogical and structural analysis [J].
Khrissi, S. ;
Bejjit, L. ;
Haddad, M. ;
Falgueres, C. ;
Lyazidi, S. Ait ;
El Amraoui, M. .
SUSTAINABLE BUILDINGS AND CITIES, 2017, 2018, 353
[15]   Raman and XRD characterization of Moroccan Marbles [J].
Khrissi, S. ;
Haddad, M. ;
Bejjit, L. ;
Lyazidi, S. Ait ;
El Aniraoui, M. ;
Falgueres, C. .
XII MAGHREB DAYS OF MATERIAL SCIENCES, 2017, 186
[16]   Monoclinic structure of unpoled morphotropic high piezoelectric PMN-PT and PZN-PT compounds [J].
Kiat, JM ;
Uesu, Y ;
Dkhil, B ;
Matsuda, M ;
Malibert, C ;
Calvarin, G .
PHYSICAL REVIEW B, 2002, 65 (06) :641061-641064
[17]   Slow dynamics and ergodicity breaking in a lanthanum-modified lead zirconate titanate relaxor system [J].
Kutnjak, Z ;
Filipic, C ;
Pirc, R ;
Levstik, A ;
Farhi, R ;
El Marssi, M .
PHYSICAL REVIEW B, 1999, 59 (01) :294-301
[18]   Glassy freezing in relaxor ferroelectric lead magnesium niobate [J].
Levstik, A ;
Kutnjak, Z ;
Filipic, C ;
Pirc, R .
PHYSICAL REVIEW B, 1998, 57 (18) :11204-11211
[19]   Effects of electrical boundary conditions and poling approaches on the mechanical depolarization behavior of PZT ceramics [J].
Li, FX ;
Fang, DN .
ACTA MATERIALIA, 2005, 53 (09) :2665-2673
[20]  
Lifi H, 2017, SENSOR LETT, V15, P751, DOI [10.1166/sl.2017.3868, 10.1166/sl.2017.3868, DOI 10.1166/SL.2017.3868]