Temperature dependent Raman and photoluminescence of vertical WS2/MoS2 monolayer heterostructures

被引:1
|
作者
Zhijian Hu [1 ]
Yanjun Bao [2 ]
Ziwei Li [2 ]
Yongji Gong [4 ]
Rui Feng [2 ]
Yingdong Xiao [2 ]
Xiaochun Wu [1 ]
Zhaohui Zhang [2 ]
Xing Zhu [2 ,1 ]
Pulickel M.Ajayan [4 ]
Zheyu Fang [2 ]
机构
[1] Key Laboratory of Nanoscale Measurement and Standardization National Center for Nanoscience and Technology
[2] State Key Laboratory for Mesoscopic Physics, School of Physics, Peking University
[3] Collaborative Innovation Center of Quantum Matter
[4] Department of Materials Science and Nano Engineering, Rice University
基金
北京市自然科学基金; 中国国家自然科学基金;
关键词
Temperature-dependent; Raman spectra; Photoluminescence; Transition metal dichalcogenides; Heterostructures;
D O I
暂无
中图分类号
TN304.2 [化合物半导体];
学科分类号
0805 ; 080501 ; 080502 ; 080903 ;
摘要
Heterostructures from two-dimensional transition-metal dichalcogenides MX2have emerged as a hot topic in recent years due to their various fascinating properties. Here, we investigated the temperature dependent Raman and photoluminescence(PL) spectra in vertical stacked WS2/MoS2monolayer heterostructures. Our result shows that both E2g1and A1gmodes of WS2and MoS2vary linearly with temperature increasing from 300 to 642 K. The PL measurement also reveals strong temperature dependencies of the PL intensity and peak position. The activation energy of the thermal quenching of the PL emission has been found to be equal to 69.6 meV. The temperature dependence of the peak energy well follows the bandgap shrinkage of bulk semiconductor.
引用
收藏
页码:16 / 21
页数:6
相关论文
共 50 条
  • [21] Tellurium-Assisted Low-Temperature Synthesis of MoS2 and WS2 Monolayers
    Gong, Yongji
    Lin, Zhong
    Ye, Gonglan
    Shi, Gang
    Feng, Simin
    Lei, Yu
    Elias, Ana Laura
    Perea-Lopez, Nestor
    Vajtai, Robert
    Terrones, Humberto
    Liu, Zheng
    Terrones, Mauricio
    Ajayan, Pulickel M.
    ACS NANO, 2015, 9 (12) : 11658 - 11666
  • [22] Anti-Stokes Photoluminescence of Monolayer WS2
    Pierret, Aurelie
    Tornatzky, Hans
    Maultzsch, Janina
    PHYSICA STATUS SOLIDI B-BASIC SOLID STATE PHYSICS, 2019, 256 (12):
  • [23] Temperature dependent photoluminescence from WS2 nanostructures
    Sharma, Shivani
    Bhagat, Shubham
    Singh, Jasvir
    Ahmad, Manzoor
    Sharma, Sandeep
    JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS, 2018, 29 (23) : 20064 - 20070
  • [24] Band Alignment in MoS2/WS2 Transition Metal Dichalcogenide Heterostructures Probed by Scanning Tunneling Microscopy and Spectroscopy
    Hill, Heather M.
    Rigosi, Albert F.
    Rim, Kwang Taeg
    Flynn, George W.
    Heinz, Tony F.
    NANO LETTERS, 2016, 16 (08) : 4831 - 4837
  • [25] Atomically Resolved Observation of Continuous Interfaces between an As-Grown MoS2 Monolayer and a WS2/MoS2 Heterobilayer on SiO2
    Zhang, Fan
    Lu, Zhixing
    Choi, Yichul
    Liu, Haining
    Zheng, Husong
    Xie, Liming
    Park, Kyungwha
    Jiao, Liying
    Tao, Chenggang
    ACS APPLIED NANO MATERIALS, 2018, 1 (05) : 2041 - 2048
  • [26] Deformation Mechanisms of Vertically Stacked WS2/MoS2 Heterostructures: The Role of Interfaces
    Susarla, Sandhya
    Manimunda, Praveena
    Jaques, Ygor Morais
    Hachtel, Jordan A.
    Idrobo, Juan Carlos
    Amnulla, Syed Asif Syed
    Galvao, Douglas Soares
    Tiwary, Chandra Sekhar
    Ajayan, Pulickel M.
    ACS NANO, 2018, 12 (04) : 4036 - 4044
  • [27] Raman and photoluminescence spectra of two-dimensional nanocrystallites of monolayer WS2 and WSe2
    Shi, Wei
    Lin, Miao-Ling
    Tan, Qing-Hai
    Qiao, Xiao-Fen
    Zhang, Jun
    Tan, Ping-Heng
    2D MATERIALS, 2016, 3 (02):
  • [28] MoS2/WS2 Heterojunction for Photoelectrochemical Water Oxidation
    Pesci, Federico M.
    Sokolikova, Maria S.
    Grotta, Chiara
    Sherrell, Peter C.
    Reale, Francesco
    Sharda, Kanudha
    Ni, Na
    Palczynski, Pawel
    Mattevi, Cecilia
    ACS CATALYSIS, 2017, 7 (08): : 4990 - 4998
  • [29] Distinguishing Ultrafast Energy Transfer in Atomically Thin MoS2/WS2 Heterostructures
    Zeng, Yan
    Dai, Wei
    Ma, Rundong
    Li, Zhe
    Ou, Zhenwei
    Wang, Cheng
    Yu, Yiling
    Zhu, Tong
    Liu, Xiaoze
    Wang, Ti
    Xu, Hongxing
    SMALL, 2022, 18 (44)
  • [30] Atomic defect states in monolayers of MoS2 and WS2
    Salehi, Saboura
    Saffarzadeh, Alireza
    SURFACE SCIENCE, 2016, 651 : 215 - 221