Emissions of parent, nitrated, and oxygenated polycyclic aromatic hydrocarbons from indoor corn straw burning in normal and controlled combustion conditions

被引:0
|
作者
Guofeng Shen [1 ,2 ]
Miao Xue [1 ,2 ]
Siye Wei [1 ]
Yuanchen Chen [1 ]
Bin Wang [1 ]
Rong Wang [1 ]
Yan Lv [1 ]
Huizhong Shen [1 ]
Wei Li [1 ]
Yanyan Zhang [1 ]
Ye Huang [1 ]
Han Chen [1 ]
Wen Wei [1 ]
Qiuyue Zhao [2 ]
Bing Li [2 ]
Haisuo Wu [2 ]
Shu Tao [1 ]
机构
[1] Laboratory of Earth Surface Processes, College of Urban and Environmental Sciences, Peking University
[2] Jiangsu Provincal Academy of Environmental Sciences
基金
中国国家自然科学基金;
关键词
polycyclic aromatic hydrocarbons; PAH derivatives; emission factor; influencing factor; indoor crop straw burning;
D O I
暂无
中图分类号
X51 [大气污染及其防治];
学科分类号
0706 ; 070602 ;
摘要
Emission factors(EFs) of parent polycyclic aromatic hydrocarbons(pPAHs), nitrated PAHs(nPAHs), and oxygenated PAHs(oPAHs)were measured for indoor corn straw burned in a brick cooking stove under diferent burning conditions. The EFs of total 28 pPAHs,6 nPAHs and 4 oPAHs were(7.9 ± 3.4),(6.5 ± 1.6)×10 3, and(6.1 ± 1.4)×10 1mg/kg, respectively. Fuel charge size had insignificant influence on the pollutant emissions. Measured EFs increased significantly in a fast burning due to the oxygen deficient atmosphere formed in the stove chamber. In both restricted and enhanced air supply conditions, the EFs of pPAHs, nPAHs and oPAHs were significantly higher than those measured in normal burning conditions. Though EFs varied among diferent burning conditions, the composition profiles and calculated isomer ratios were similar, without significant diferences. The results from the stepwise regression model showed that fuel burning rate, air supply amount, and modified combustion efciency were the three most significant influencing factors, explaining 72%–85% of the total variations.
引用
收藏
页码:2072 / 2080
页数:9
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