Creation of passivated Nb/N p-n co-doped ZnO nanoparticles and their enhanced photocatalytic performance under visible light illumination
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作者:
Shuang Gao
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机构:
Division of Energy and Environment,Graduate School at Shenzhen,Tsinghua UniversityDivision of Energy and Environment,Graduate School at Shenzhen,Tsinghua University
Shuang Gao
[1
]
Weiyi Yang
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机构:
Environment Functional Materials Division,Shenyang National Laboratory for Materials Science,Institute of Metal Research,Chinese Academy of SciencesDivision of Energy and Environment,Graduate School at Shenzhen,Tsinghua University
Weiyi Yang
[2
]
Jun Xiao
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机构:
Environment Functional Materials Division,Shenyang National Laboratory for Materials Science,Institute of Metal Research,Chinese Academy of SciencesDivision of Energy and Environment,Graduate School at Shenzhen,Tsinghua University
Jun Xiao
[2
]
Bo Li
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机构:
Division of Energy and Environment,Graduate School at Shenzhen,Tsinghua UniversityDivision of Energy and Environment,Graduate School at Shenzhen,Tsinghua University
Bo Li
[1
]
Qi Li
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机构:
Environment Functional Materials Division,Shenyang National Laboratory for Materials Science,Institute of Metal Research,Chinese Academy of SciencesDivision of Energy and Environment,Graduate School at Shenzhen,Tsinghua University
Qi Li
[2
]
机构:
[1] Division of Energy and Environment,Graduate School at Shenzhen,Tsinghua University
[2] Environment Functional Materials Division,Shenyang National Laboratory for Materials Science,Institute of Metal Research,Chinese Academy of Sciences
Passivated niobium/nitrogen(Nb-N) p-n co-doped zinc oxide nanoparticles were created by a simple precipitation process with in-situ self-formed NaCl "cage" to confine the nanoparticle growth followed by the heat treatment in a flow of ammonia gas. Enhanced optical absorbance into the visible light region was observed in the Nb/N co-doped ZnO nanoparticle photocatalyst due to the Nb/N co-doping effect.It demonstrated a largely enhanced photocatalytic performance in the disinfection of Escherichia coli bacteria under visible light illumination, which could be attributed to the passivated co-doping of NbN to suppress the photogenerated charge carrier recombination on dopants. This robust approach for passivated p-n co-doping may also be applied to other material systems for a wide range of technical applications.