Synthesis,photophysical properties and TD-DFT calculation of four two-photon absorbing triphenylamine derivatives

被引：0

作者：

KONG Lin ^{[1
]}

YANG JiaXiang ^{[1
,2
]}

ZHOU HongPing ^{[1
]}

LI ShengLi ^{[1
]}

HAO FuYing ^{[1
]}

ZHANG Qiong ^{[1
]}

TU YuLong ^{[1
]}

WU JieYing ^{[1
]}

XUE ZhaoMing ^{[1
]}

TIAN YuPeng ^{[1
,2
,3
]}

机构：

[1] Department of Chemistry,Key Laboratory of Functional Inorganic Materials of Anhui Province,Anhui University

[2] State Key Laboratory of Crystal Materials,Shandong University

[3] State Key Laboratory of Coordination Chemistry,Nanjing University

来源：

Science China(Chemistry) | 2013年 / 01期

关键词：

triphenylamine derivatives; optical properties; structure-property relationship; TD-DFT calculation;

D O I：

暂无

中图分类号：

O625.631 [];

学科分类号：

070303 ; 081704 ;

摘要：

In this study,linear absorption,single-photon excited fluorescence,fluorescence quantum yields,fluorescence lifetime and two-photon excited fluorescence of a series of triphenylamine derivatives (L1,L2,L3 and L4) have been measured.L1 and L3 are D--A type dyes,while L2 and L4 are D--D--A type dyes (D=donor,A=acceptor).The investigated compounds consist of triphenylamine-bearing donor-substituted and/or systematically extended-conjugated length,which are designed to gain insight into the effect of the ethoxyl unit and-linkage length on the linear and nonlinear optical properties.The influence of solvent polarity on the photophysical properties was investigated.Employing time-dependent density functional theory (TD-DFT) calculations,the structure-property relationships are discussed.

引用

页码：106 / 116

页数：11

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