Fe–N–C电催化氧还原反应催化剂的研究进展(英文)

被引:10
作者
王颖 [1 ]
王蕾 [2 ]
付宏刚 [2 ]
机构
[1] Key Laboratory of Superlight Materials and Surface Technology of Ministry of Education, College of Materials Science and Chemical Engineering, Harbin Engineering University
[2] Key Laboratory of Functional Inorganic Material Chemistry, Ministry of Education of China, Heilongjiang
关键词
D O I
暂无
中图分类号
O643.36 [催化剂]; TM911.4 [燃料电池];
学科分类号
摘要
氧还原反应(ORR)是燃料电池和金属-空气电池等各种能源转换器件中重要的半反应.由于ORR的动力学缓慢,需要开发高活性电催化剂来替代常用的贵金属铂基催化剂. Fe-N-C催化剂被认为是最有前景的材料,其丰富的活性位点可以降低含氧中间体的能垒.在这篇综述中,我们详细总结了Fe-N-C催化剂在理论和实验研究方面的最新研究进展.首先,概述了基于Fe-N-C催化剂的电催化ORR的反应机理.然后,对Fe-N-C催化剂的设计策略和活性位点进行了分类.接下来,讨论了活性位点与催化性能之间的关系.介绍了Fe-N-C催化剂在燃料电池和锌空气电池中的应用现状.最后,进一步提出了Fe-N-C催化剂在可控合成、机理研究和能源器件应用方面面临的挑战和机遇.
引用
收藏
页码:1701 / 1722
页数:22
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