A Numerical Study of Tropospheric Ozone in the Springtime in East Asia

被引:0
作者
张美根
徐永福
Itsushi UNO
Hajime AKIMOTO
机构
[1] Beijing 100029
[2] Chinese Academy of Sciences
[3] Frontier Research System for Global Change
[4] Institute of Atmospheric Physics
[5] Japan
[6] Kanagawa 236-0001
[7] Kasuga 816-8580
[8] Kasuga Park 6-1
[9] Research Institute for Applied Mechanics of Kyushu University
[10] State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry
[11] Yokohama
关键词
regional pollution; tropospheric ozone; carbon monoxide; Community Multi-scale Air Quality modeling system;
D O I
暂无
中图分类号
P421.3 [大气结构];
学科分类号
0706 ; 070601 ;
摘要
The Models-3 Community Multi-scale Air Quality modeling system (CMAQ) coupled with the Regional Atmospheric Modeling System (RAMS) is applied to East Asia to study the transport and photochemical transformation of tropospheric ozone in March 1998. The calculated mixing ratios of ozone and carbon monoxide are compared with ground level observations at three remote sites in Japan and it is found that the model reproduces the observed features very well. Examination of several high episodes of ozone and carbon monoxide indicates that these elevated levels are found in association with continental outflow, demonstrating the critical role of the rapid transport of carbon monoxide and other ozone precursors from the continental boundary layer. In comparison with available ozonesonde data, it is found that the model-calculated ozone concentrations are generally in good agreement with the measurements, and the stratospheric contribution to surface ozone mixing ratios is quite limited.
引用
收藏
页码:163 / 170
页数:8
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