Scale-Up Synthesis of Hydrogen Peroxide from H2/O2 with Multiple Parallel DBD Tubes

被引:0
作者
赵剑利 [1 ]
周军成 [1 ]
苏际 [1 ]
郭洪臣 [1 ]
王祥生 [1 ]
宫为民 [1 ]
机构
[1] Department of Catalytic Chemistry and Engineering & State Key Laboratory of Fine Chemicals Dalian University of Technology
基金
中国国家自然科学基金;
关键词
hydrogen peroxide; non-equilibrium plasma; scale-up; parallel DBD tubes;
D O I
暂无
中图分类号
O461.2 [各类型放电];
学科分类号
0809 ; 080901 ;
摘要
The scale-up synthesis of HOfrom HOvia a dielectric barrier discharge(DBD)under ambient conditions was studied.A plasma reactor consisting of multiple parallel DBDtubes was designed to scale up the HOsynthesis.The number of tubes had no significant effecton the discharge mode,and no decay occurred in HOselectivity during the scale-up process.These advantages made this technology more stable and efficient.The reactor’s energy efficiencyincreased with the number of tubes and reached 136 g HO/kWh in the four-tube reaction.Thetotal energy efficiency was limited by the extremely low energy transfer efficiency of power supply,and might be enhanced by optimizing the impedance matching between the power supply and thereactor load.As a result,an assembly of multiple DBD tubes may provide a viable route for thescale-up synthesis of HOby a non-equilibrium plasma.
引用
收藏
页码:181 / 186
页数:6
相关论文
共 50 条
  • [21] Direct synthesis of hydrogen peroxide using concentrated H2 and O2 mixtures in a wall-coated microchannel - kinetic study
    Paunovic, Violeta
    Schouten, Jaap C.
    Nijhuis, T. Alexander
    APPLIED CATALYSIS A-GENERAL, 2015, 505 : 249 - 259
  • [22] Direct Synthesis of H2O2 by a H2/O2 Fuel Cell
    Ichiro Yamanaka
    Catalysis Surveys from Asia, 2008, 12 : 78 - 87
  • [23] Direct synthesis of H2O2 by a H2/O2 fuel cell
    Yamanaka, Ichiro
    CATALYSIS SURVEYS FROM ASIA, 2008, 12 (02) : 78 - 87
  • [24] Direct formation of H2O2 from H2 and O2
    Yildiz, Meltem
    Akin, Ayse Nilguen
    TURKISH JOURNAL OF CHEMISTRY, 2007, 31 (05) : 479 - 486
  • [25] The Promotion of Argon and Water Molecule on Direct Synthesis of H2O2 from H2 and O2
    Yi, Yanhui
    Wang, Li
    Yu, Juan
    Guo, Hongchen
    Zhang, Jialiang
    Meng, Changgong
    AICHE JOURNAL, 2018, 64 (03) : 981 - 992
  • [26] Safe Direct Synthesis of High Purity H2O2 through a H2/O2 Plasma Reaction
    Yi, Yanhui
    Zhou, Juncheng
    Guo, Hongchen
    Zhao, Jianli
    Su, Ji
    Wang, Li
    Wang, Xiangsheng
    Gong, Weimin
    ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2013, 52 (32) : 8446 - 8449
  • [27] Catalytic Synthesis of Neutral H2O2 Solutions from O2 and H2 by a Fuel Cell Reaction
    Yamanaka, Ichiro
    Tazawa, Satoshi
    Murayama, Toru
    Ichihashi, Ryo
    Hanaizumi, Noriko
    CHEMSUSCHEM, 2008, 1 (12) : 988 - 992
  • [28] Direct and Safe Synthesis of H2O2 from O2 and H2 Using Fuel Cell Reactors
    Yamanaka, Ichiro
    JOURNAL OF THE JAPAN PETROLEUM INSTITUTE, 2014, 57 (06) : 237 - 250
  • [29] SBA-15 as a support for palladium in the direct synthesis of H2O2 from H2 and O2
    Abate, S.
    Lanzafame, P.
    Perathoner, S.
    Centi, G.
    CATALYSIS TODAY, 2011, 169 (01) : 167 - 174
  • [30] In Situ Mapping of H2, O2, and H2O2 in Microreactors: A Parallel, Selective Multianalyte Detection Method
    Urban, Sebastian
    Deschner, Benedikt J.
    Trinkies, Laura L.
    Kieninger, Jochen
    Kraut, Manfred
    Dittmeyer, Roland
    Urban, Gerald A.
    Weltin, Andreas
    ACS SENSORS, 2021, 6 (04) : 1583 - 1594