Atmospheric Pressure Glow Discharge in a Mixture of Carbon Dioxide and Methane

被引:0
作者
Batukaev, Timur [1 ]
Epstein, Irene [1 ]
Lebedev, Yuri [1 ]
机构
[1] AV Topchiev Inst Petrochem Synth Russian Acad Sci, Moscow, Russia
关键词
CO2; decomposition; dry reforming; glow discharge; hydrogen production; low temperature plasma; HYDROGEN-PRODUCTION; ROTATIONAL TEMPERATURES; DECOMPOSITION; CONVERSION; OH;
D O I
10.1002/ppap.70043
中图分类号
O59 [应用物理学];
学科分类号
摘要
The electrical characteristics, emission spectra, and composition of gas products in a DC discharge mixture of CO2 and CH4 at different polarities of the applied voltage and an AC discharge (50 Hz) at atmospheric pressure and different ratios of CO2 and CH4 flow rates have been investigated. The best degree of CH4 decomposition is about 95%. The degree of CO2 decomposition ranges from 85%-95% at a CO2/CH4 consumption ratio equal to one. The best characteristics of the decomposition process are obtained in a direct current discharge under conditions when the cathode is located in the part of the discharge tube opposite to the point of introduction of the gas mixture.
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页数:11
相关论文
共 45 条
[31]   Non-thermal plasma approaches in CO2 utilization [J].
Liu, CJ ;
Xu, GH ;
Wang, TM .
FUEL PROCESSING TECHNOLOGY, 1999, 58 (2-3) :119-134
[32]   A review on coke management during dry reforming of methane [J].
Muraza, Oki ;
Galadima, Ahmad .
INTERNATIONAL JOURNAL OF ENERGY RESEARCH, 2015, 39 (09) :1196-1216
[33]   A comparative overview of hydrogen production processes [J].
Nikolaidis, Pavlos ;
Poullikkas, Andreas .
RENEWABLE & SUSTAINABLE ENERGY REVIEWS, 2017, 67 :597-611
[34]  
Nozaki T, 2019, SPRINGER SER ATOM OP, V106, P231, DOI 10.1007/978-3-030-05189-1_8
[35]   Greenhouse gas treatment and H2 production, by warm plasma reforming [J].
Pacheco, J. ;
Soria, G. ;
Pacheco, M. ;
Valdivia, R. ;
Ramos, F. ;
Frias, H. ;
Duran, M. ;
Hidalgo, M. .
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2015, 40 (48) :17165-17171
[36]   Methane conversion in low-temperature plasma [J].
Pushkarev, A. I. ;
Zhu, Ai-Min ;
Li, Xiao-Song ;
Sazonov, R. V. .
HIGH ENERGY CHEMISTRY, 2009, 43 (03) :156-162
[37]  
Raizer Y.P., 1991, GAS DISCHARGE PHYS, VVolume 1
[38]   Rotational temperatures of N2(C,0) and OH(A,0) as gas temperature estimates in the middle pressure Ar/O2 discharge [J].
Raud, J. ;
Laan, M. ;
Jogi, I. .
JOURNAL OF PHYSICS D-APPLIED PHYSICS, 2011, 44 (34)
[39]   State of the Art of Hydrogen Production via Pyrolysis of Natural Gas [J].
Schneider, Stefan ;
Bajohr, Siegfried ;
Graf, Frank ;
Kolb, Thomas .
CHEMBIOENG REVIEWS, 2020, 7 (05) :150-158
[40]  
Sheng Z., 2018, Book: Plasma Chemistry and Gas Conversion, DOI [10.5772/intechopen.80523, DOI 10.5772/INTECHOPEN.80523]