Long-lived coherence between incoherent excitons revealed by time-resolved angle-resolved photoemission spectroscopy: An exact solution

被引：0

作者：

Zhang, Zhenlin ^{[1
]}

Hu, Wei ^{[1
]}

Perfetto, Enrico ^{[2
,3
]}

Stefanucci, Gianluca ^{[2
,3
]}

机构：

[1] Univ Sci & Technol China, Hefei Natl Res Ctr Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China

[2] Univ Roma Tor Vergata, Dipartimento Fis, Via Ric Sci 1, I-00133 Rome, Italy

[3] Inst Nazl Fis Nucl, Sez Roma Tor Vergata, Via Ric Sci 1, I-00133 Rome, Italy

来源：

PHYSICAL REVIEW B | 2025年 / 111卷 / 23期

基金：

欧洲研究理事会;

关键词：

BLOCH EQUATIONS; DYNAMICS;

D O I：

10.1103/9spx-3hrq

中图分类号：

T [工业技术];

学科分类号：

08 ;

摘要：

We investigate the exciton dynamics in an exactly solvable two-band model for semiconductors. The model incorporates light-matter, electron-electron, and electron-phonon interactions, and captures exciton formation as well as the transition from the coherent to the incoherent regime. We analyze excitonic polarization, populations, and coherences, with special focus on their impact in time-resolved angle-resolved photoemission spectroscopy (TR-ARPES). For nonresonant pumping with below-gap photon energies, TR-ARPES spectra reveal distinct excitonic replica and quantum beats persisting in the incoherent regime. These are due to a coherence between different species of incoherent excitons. Such type of coherence is resistant to phonon dephasing, indicating that it follows different dynamics than those governing the coherences considered so far.

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页数：16

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