Soft X-ray photoelectron spectroscopy under real ambient pressure conditions

被引:0
作者
Wada, Tetsuya [1 ]
Horio, Masafumi [1 ]
Liu, Yifu [1 ]
Murano, Yu [1 ]
Sakurai, Haruto [1 ]
Sumi, Toshihide [1 ]
Miyamoto, Masashige [1 ]
Yamamoto, Susumu [2 ,3 ]
Matsuda, Iwao [1 ,2 ]
机构
[1] Univ Tokyo, Inst Solid State Phys ISSP, Kashiwa, Chiba 2778581, Japan
[2] Tohoku Univ, Int Ctr Synchrotron Radiat Innovat Smart SRIS, Sendai, Miyagi 9808577, Japan
[3] Tohoku Univ, Inst Multidisciplinary Res Adv Mat IMRAM, Sendai, Miyagi 9808577, Japan
基金
日本学术振兴会;
关键词
ambient pressure X-ray photoelectron spectroscopy; surface; soft X-ray; synchrotron radiation; X-ray photoelectron spectroscopy; operando measurement; gas/solid interface; SCATTERING CROSS-SECTIONS; ELECTRON-SCATTERING; CO2;
D O I
10.35848/1882-0786/adbda8
中图分类号
O59 [应用物理学];
学科分类号
摘要
We have developed a measurement system for soft X-ray ambient pressure photoelectron spectroscopy at BL08U of NanoTerasu. An excitation light of 800 eV was introduced by a vacuum tube terminated with a SiN window. Photoelectrons were detected through a phi 24 mu m aperture at the electron lens entrance of a differentially pumped analyzer. The Au 4f core-level spectra of a Au film were measured up to atmospheric pressure (1 bar) with He, to 1 bar with H2, and to 0.4 bar with N2. The system extends applications of operando experiments for the real functional materials.
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页数:4
相关论文
共 33 条
[1]   A high-pressure x-ray photoelectron spectroscopy instrument for studies of industrially relevant catalytic reactions at pressures of several bars [J].
Amann, Peter ;
Degerman, David ;
Lee, Ming-Tao ;
Alexander, John D. ;
Shipilin, Mikhail ;
Wang, Hsin-Yi ;
Cavalca, Filippo ;
Weston, Matthew ;
Gladh, Jorgen ;
Blom, Mikael ;
Bjorkhage, Mikael ;
Lofgren, Patrik ;
Schlueter, Christoph ;
Loemker, Patrick ;
Ederer, Katrin ;
Drube, Wolfgang ;
Noei, Heshmat ;
Zehetner, Johann ;
Wentzel, Henrik ;
Ahlund, John ;
Nilsson, Anders .
REVIEW OF SCIENTIFIC INSTRUMENTS, 2019, 90 (10)
[2]   Lab-based ambient pressure X-ray photoelectron spectroscopy from past to present [J].
Arble, Chris ;
Jia, Meng ;
Newberg, John T. .
SURFACE SCIENCE REPORTS, 2018, 73 (02) :37-57
[3]   Total electron scattering cross sections of He, Ne and Ar at intermediate electron energies [J].
Ariyasinghe, WM ;
Goains, C ;
Powers, D ;
Wijeratne, T ;
Palihawadana, P .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS, 2004, 225 (03) :191-197
[4]   Photoelectron spectroscopy of surfaces under humid conditions [J].
Bluhm, Hendrik .
JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA, 2010, 177 (2-3) :71-84
[5]   In situ near-ambient pressure X-ray photoelectron spectroscopy discloses the surface composition of operating NdBaCo2O5+δ solid oxide fuel cell cathodes [J].
Bozzini, Benedetto ;
Previdi, Anita ;
Amati, Matteo ;
Bevilacqua, Manuela ;
Cordaro, Giulio ;
Corva, Manuel ;
Donazzi, Alessandro ;
Dotelli, Giovanni ;
Gregoratti, Luca ;
Pelosato, Renato ;
Vorokhta, Mykhailo ;
Vesselli, Erik .
JOURNAL OF POWER SOURCES, 2019, 436
[6]   NAP-XPS Probes the Electronic Structure of the Mg-Al-Cl Layered Double Hydroxide upon Controlled Hydration [J].
Coustel, Romain ;
Boucly, Anthony ;
Andre, Erwan ;
Di Bitetto, Arnaud ;
Bournel, Fabrice ;
Gallet, Jean-Jacques ;
Rochet, Francois ;
Carteret, Cedric .
JOURNAL OF PHYSICAL CHEMISTRY C, 2023, 127 (08) :4144-4153
[7]   TOTAL CROSS-SECTION FOR ELECTRON-SCATTERING FROM N-2 IN THE ENERGY-RANGE 600-5000 EV [J].
GARCIA, G ;
PEREZ, A ;
CAMPOS, J .
PHYSICAL REVIEW A, 1988, 38 (02) :654-657
[8]   Operando probing of the surface chemistry during the Haber-Bosch process [J].
Goodwin, Christopher M. ;
Lomker, Patrick ;
Degerman, David ;
Davies, Bernadette ;
Shipilin, Mikhail ;
Garcia-Martinez, Fernando ;
Koroidov, Sergey ;
Mathiesen, Jette Katja ;
Rameshan, Raffael ;
Rodrigues, Gabriel L. S. ;
Schlueter, Christoph ;
Amann, Peter ;
Nilsson, Anders .
NATURE, 2024, 625 (7994) :282-286
[9]   X-RAY INTERACTIONS - PHOTOABSORPTION, SCATTERING, TRANSMISSION, AND REFLECTION AT E=50-30,000 EV, Z=1-92 [J].
HENKE, BL ;
GULLIKSON, EM ;
DAVIS, JC .
ATOMIC DATA AND NUCLEAR DATA TABLES, 1993, 54 (02) :181-342
[10]  
Hufner S., 2013, PHOTOELECTRON SPECTR