Synergistic effects of magnetic fields and flow velocity on hydrogen bubble dynamics in water electrolysis

被引:0
作者
Sun, Jindong [1 ]
Wang, Caizhu [1 ]
Wen, Haoyu [1 ]
Yin, Qian [1 ]
Fan, Jiaci [1 ]
机构
[1] Beijing Univ Civil Engn & Architecture, Sch Environm & Energy Engn, Beijing 100044, Peoples R China
关键词
Magnetic field; Flow velocity; Electrochemical reaction; Hydrogen bubble dynamics; Hydrogen evolution reaction (HER); EXCHANGE MEMBRANE ELECTROLYZER; 2-PHASE FLOW; GAS-BUBBLES; CONVECTION; DETACHMENT; LORENTZ; SURFACE; GROWTH; MICROELECTRODE; PERFORMANCE;
D O I
10.1016/j.elecom.2025.107918
中图分类号
O646 [电化学、电解、磁化学];
学科分类号
081704 ;
摘要
By systematically regulating the magnetic field intensity and electrolyte flow rate, this study investigates the coupling effects of magnetic fields and flow velocity on hydrogen bubble dynamics during water electrolysis. A model of hydrogen bubble dynamics was used to analyze nucleation, growth, and detachment mechanisms under magnetic-flow coupling, determining key parameters such as growth radius and detachment speed. The dynamic evolution of hydrogen bubbles was comprehensively analyzed under both static and dynamic flow conditions. Electrochemical measurements revealed that increasing the magnetic field intensity from 0 T to 0.3 T enhanced the current density by 9.61 % at 0 cm/s and 6.67 % at 1 cm/s flow rates. These results suggest that magnetic-flow coupling reduces concentration polarization and overpotential. However, the enhancement effect gradually diminished with increasing flow velocity. Visualization experiments further confirmed that the coupling between magnetic field and flow velocity significantly promoted bubble oscillation, coalescence, and detachment, thereby improving electrolysis performance.
引用
收藏
页数:15
相关论文
共 83 条
  • [31] Investigation of alkaline water electrolysis performance for different cost effective electrodes under magnetic field
    Kaya, Mehmet Fatih
    Demir, Nesrin
    Albawabiji, M. Salahaldin
    Tas, Mert
    [J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2017, 42 (28) : 17583 - 17592
  • [32] Effects of bubbles on the electrochemical behavior of hydrogen-evolving Si microwire arrays oriented against gravity
    Kempler, Paul A.
    Coridan, Robert H.
    Lewis, Nathan S.
    [J]. ENERGY & ENVIRONMENTAL SCIENCE, 2020, 13 (06) : 1808 - 1817
  • [33] Kiros Y, 2008, INT J ELECTROCHEM SC, V3, P444
  • [34] Analysis of gas dissociation rate into liquid phase under magnetic field gradient
    Kishioka, S
    Yamada, A
    Aogaki, R
    [J]. PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2000, 2 (18) : 4179 - 4183
  • [35] Magnetic field effects on water, air and powders
    Kitazawa, K
    Ikezoe, Y
    Uetake, H
    Hirota, N
    [J]. PHYSICA B, 2001, 294 : 709 - 714
  • [36] VAPOR BUBBLE DEPARTURE IN FORCED-CONVECTION BOILING
    KLAUSNER, JF
    MEI, R
    BERNHARD, DM
    ZENG, LZ
    [J]. INTERNATIONAL JOURNAL OF HEAT AND MASS TRANSFER, 1993, 36 (03) : 651 - 662
  • [37] Hydrogen evolution under the influence of a magnetic field
    Koza, Jakub Adam
    Muehlenhoff, Sascha
    Zabinski, Piotr
    Nikrityuk, Petr A.
    Eckert, Kerstin
    Uhlemann, Margitta
    Gebert, Annett
    Weier, Tom
    Schultz, Ludwig
    Odenbach, Stefan
    [J]. ELECTROCHIMICA ACTA, 2011, 56 (06) : 2665 - 2675
  • [38] Entropy Generation Due to the Heat Transfer for Evolving Spherical Objects
    Kwak, Ho-Young
    [J]. ENTROPY, 2018, 20 (08):
  • [39] Efficient Mesh Interface Engineering: Insights from Bubble Dynamics in Electrocatalysis
    Li, Long
    Jiang, Wenjun
    Zhang, Guang
    Feng, Deqiang
    Zhang, Ce
    Yao, Wei
    Wang, Zhijie
    [J]. ACS APPLIED MATERIALS & INTERFACES, 2021, 13 (38) : 45346 - 45354
  • [40] The effect of magnetic field on the dynamics of gas bubbles in water electrolysis
    Li, Yan-Hom
    Chen, Yen-Ju
    [J]. SCIENTIFIC REPORTS, 2021, 11 (01)