Direct air capture (DAC): molten carbonate direct transformation of airborne CO2 to durable, useful carbon nanotubes and nano-onions

被引:0
|
作者
Licht, Gad [1 ]
Peltier, Ethan [2 ]
Gee, Simon [2 ]
Licht, Stuart [1 ,2 ,3 ]
机构
[1] Direct Air Capture LLC, A4 188 Triple Diamond Blvd, North Venice, FL 34275 USA
[2] Carbon Corp, 1035 26 St NE, Calgary, AB T2A 6K8, Canada
[3] George Washington Univ, Dept Chem, Washington, DC 20052 USA
来源
RSC SUSTAINABILITY | 2025年 / 3卷 / 03期
关键词
ELECTROLYSIS; DIOXIDE;
D O I
10.1039/d4su00679h
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
This study introduces the concept and first demonstration of an effective molten carbonate chemistry for Direct Air Capture (DAC). Molten carbonate electrolysis is a high-temperature decarbonization process within Carbon Capture, Utilization and Storage (CCUS) that transforms chemistry transforming flue gas CO2 into carbon nanotubes and carbon nano-onions. The key challenge for molten carbonate DAC is to split air's 0.04% CO2 without heating the remaining 99.6%. This is accomplished by integrating a diffusive, insulating membrane over an electrolyte with a high affinity for CO2.
引用
收藏
页码:1339 / 1345
页数:7
相关论文
共 26 条
  • [21] Direct electrolytic dissolution of silicate minerals for air CO2 mitigation and carbon-negative H2 production
    Rau, Greg H.
    Carroll, Susan A.
    Bourcier, William L.
    Singleton, Michael J.
    Smith, Megan M.
    Aines, Roger D.
    PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2013, 110 (25) : 10095 - 10100
  • [22] Electrochemical direct CO2 capture technology using redox-active organic molecules to achieve carbon-neutrality
    Choi, Gwan Hyun
    Song, Hyun Jun
    Lee, Seolhwa
    Kim, Jeong Yoon
    Moon, Myoung-Woon
    Yoo, Pil J.
    NANO ENERGY, 2023, 112
  • [23] Direct, efficient and selective capture of low concentration of CO2 from natural gas flue gas using a high temperature tubular carbon capture membrane
    Sun, Shichen
    Billings, Aidan
    Zhang, Kangkang
    Huang, Kevin
    JOURNAL OF MEMBRANE SCIENCE, 2022, 661
  • [24] Direct Synthesis of Carbon Nanotubes from Only CO2 by a Hybrid Reactor of Dielectric Barrier Discharge and Solid Oxide Electrolyser Cell
    Mori, Shinsuke
    Matsuura, Naoki
    Tun, Lin Lin
    Suzuki, Masaaki
    PLASMA CHEMISTRY AND PLASMA PROCESSING, 2016, 36 (01) : 231 - 239
  • [25] Direct growth of carbon nanotubes on Ni/TiO2 as next generation catalysts for photoreduction of CO2 to methane by water under visible light irradiation
    Ong, Wee-Jun
    Gui, Meei Mei
    Chai, Siang-Piao
    Mohamed, Abdul Rahman
    RSC ADVANCES, 2013, 3 (14): : 4505 - 4509
  • [26] A new kind CO2/CH4 separation material: open ended nitrogen doped carbon nanotubes formed by direct pyrolysis of metal organic frameworks
    Shen, Yongming
    Bai, Junfeng
    CHEMICAL COMMUNICATIONS, 2010, 46 (08) : 1308 - 1310