Highly permeable anti-pollution separation membranes inspired by soil purification functions for efficient separation of dye/salt

被引:1
作者
Ma, Wensong [1 ]
Yang, Xu [1 ,2 ]
Lin, Ligang [1 ]
Li, Hongchao [1 ]
Shang, Huiyang [1 ]
Wu, Hao [1 ]
Hou, Mengfan [1 ]
Guo, Zining [1 ]
Liu, Zitian [1 ]
Yang, Jing [1 ]
Li, Bowen [3 ]
机构
[1] Tiangong Univ, Natl Ctr Int Joint Res Separat Membrane, Sch Mat Sci & Engn, State Key Lab Separat Membranes & Membrane Proc, Tianjin 300387, Peoples R China
[2] Sinopec Shengli Oilfield Water Supply Co, Dongying 257000, Peoples R China
[3] Tianjin Univ, Sch Chem Engn & Technol, Tianjin 300350, Peoples R China
基金
中国国家自然科学基金;
关键词
Polyimide membrane; Montmorillonite; Dye/salt separation; Antifouling; NANOFILTRATION MEMBRANES; MONTMORILLONITE; NANOCOMPOSITE; SELECTIVITY; FABRICATION; NANOSHEETS; REMOVAL; FLUX;
D O I
10.1016/j.memsci.2025.123937
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
The development of high-efficiency separation membranes is expected to realize the recycling of sustainable resources. It is important in separating dye/salt mixtures in textile wastewater, which can be separated by membrane separation technology to realize the reuse of dyes and salts. However, conventional membrane processes were generally constrained by the presence of fouling as well as energy and cost. The development of low-cost and high-performance separation membranes was particularly critical. Inspired by the fact that pollutants are absorbed and filtered by the soil, allowing the water to be purified. Low-cost and easily available montmorillonite (MMT) was selected and acid-modified to obtain AA-CMMT with large specific surface and pore structure. Preparation of polyimide (PI) membranes by blending AA-CMMT with membrane materials. AACMMT not only provides a water transport channel during separation, but also effectively reduces the attraction between the membrane surface and the contaminants. Improved membrane contamination resistance. Maintains high water permeability (above 110 L m(- 2) h(-1)& sdot;bar(- 1)), dye retention (>98 %), and inorganic salt retention (<20 %) in long-term separation of dye/salt wastewater. This work provides a strategy for combining naturally low-priced soils with separation membranes, which has significant potential in wastewater treatment.
引用
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页数:12
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共 80 条
[1]   High-performance mixed-matrix membranes enabled by organically/inorganic modified montmorillonite for the treatment of hazardous textile wastewater [J].
Abdel-Karim, Ahmed ;
El-Naggar, Mehrez E. ;
Radwan, E. K. ;
Mohamed, Ibrahim M. ;
Azaam, Mohamed ;
Kenawy, El-Refaie .
CHEMICAL ENGINEERING JOURNAL, 2021, 405
[2]   Purification of crude oil contaminated water using fly ash/clay [J].
Adams, F. V. ;
Peter, A. ;
Joseph, I. V. ;
Sylvester, O. P. ;
Mulaba-Bafubiandi, A. F. .
JOURNAL OF WATER PROCESS ENGINEERING, 2019, 30
[3]   A comparative study between MMT-Fe3O4/PES, MMT-HBE/PES, and MMT-acid activated/PES mixed matrix membranes [J].
Balkanloo, Peyman Gozali ;
Mahmoudian, Mehdi ;
Hosseinzadeh, Mohammad Taghi .
CHEMICAL ENGINEERING JOURNAL, 2020, 396
[4]   A Self-Cleaning Heterostructured Membrane for Efficient Oil-in-Water Emulsion Separation with Stable Flux [J].
Cai, Yahui ;
Chen, Dongyun ;
Li, Najun ;
Xu, Qingfeng ;
Li, Hua ;
He, Jinghui ;
Lu, Jianmei .
ADVANCED MATERIALS, 2020, 32 (25)
[5]   Bioapplication of cyclodextrin-containing montmorillonite [J].
Cao, Shuai ;
Liu, Chang ;
Zhou, Le ;
Zhang, Huacheng ;
Zhao, Yuxin ;
Liu, Zhaona .
JOURNAL OF MATERIALS CHEMISTRY B, 2021, 9 (45) :9241-9261
[6]   Effect of reactive montmorillonite with amino on the properties of polyimide/montmorillonite nanocomposite [J].
Chen, Shiwei ;
Xie, Jixun ;
Yang, Zhizhou .
POLYMER BULLETIN, 2020, 77 (02) :687-699
[7]   Antibacterial polyvinyl alcohol nanofiltration membrane incorporated with Cu(OH)2 nanowires for dye/salt wastewater treatment [J].
Chen, Yingdong ;
Sun, Rongze ;
Yan, Wentao ;
Wu, Mengyao ;
Zhou, Yong ;
Gao, CongJie .
SCIENCE OF THE TOTAL ENVIRONMENT, 2022, 817
[8]   Fireproof ultrastrong all-natural cellulose nanofiber/montmorillonite-supported MXene nanocomposites with electromagnetic interference shielding and thermal management multifunctional applications [J].
Cheng, Rui ;
Wu, Ying ;
Wang, Bin ;
Zeng, Jinsong ;
Li, Jinpeng ;
Xu, Jun ;
Gao, Wenhua ;
Chen, Kefu .
JOURNAL OF MATERIALS CHEMISTRY A, 2023, 11 (34) :18323-18335
[9]   The mutualism of strategic environmental assessment and sustainable development goals [J].
Del Campo, Ainhoa Gonzalez ;
Gazzola, Paola ;
Onyango, Vincent .
ENVIRONMENTAL IMPACT ASSESSMENT REVIEW, 2020, 82
[10]   High-Performance PEBA2533-Functional MMT Mixed Matrix Membrane Containing High-Speed Facilitated Transport Channels for CO2/N2 Separation [J].
Dong, Liangliang ;
Zhang, Chunfang ;
Bai, Yunxiang ;
Shi, Dongjian ;
Li, Xiaojie ;
Zhang, Hongji ;
Chen, Mingqing .
ACS SUSTAINABLE CHEMISTRY & ENGINEERING, 2016, 4 (06) :3486-3496