Recent Advances on Two-Dimensional Nanomaterials Supported Single-Atom for Hydrogen Evolution Electrocatalysts

被引:2
作者
Fu, Kangkai [1 ,2 ]
Yuan, Douke [1 ,2 ]
Yu, Ting [1 ,2 ]
Lei, Chaojun [3 ]
Kou, Zhenhui [4 ]
Huang, Bingfeng [1 ,2 ]
Lyu, Siliu [1 ,2 ]
Zhang, Feng [1 ,2 ]
Wan, Tongtao [1 ,2 ]
机构
[1] Hubei Univ Automot Technol, Sch Automot Engn, Hubei Key Lab Automot Power Train & Elect Control, Shiyan 442002, Peoples R China
[2] Hubei Univ Automot Technol, Sch Math Phys & Optoelect Engn, Hubei Key Lab Energy Storage & Power Battery, Shiyan 442002, Peoples R China
[3] Hangzhou Normal Univ, Coll Mat Chem & Chem Engn, Key Lab Organosilicon Chem & Mat Technol, Minist Educ, Hangzhou 311121, Peoples R China
[4] Zhejiang Univ, Coll Chem & Biol Engn, Key Lab Biomass Chem Engn, Minist Educ, Hangzhou 310027, Peoples R China
来源
MOLECULES | 2024年 / 29卷 / 18期
基金
中国国家自然科学基金;
关键词
two-dimensional materials; single-atom catalysts; electrocatalytic; hydrogen evolution reaction; metal-support interactions; METAL-ORGANIC FRAMEWORK; HIGH-INDEX FACETS; OXYGEN REDUCTION; MOS2; NANOSHEETS; PERFORMANCE; CATALYSIS; SIZE; CLUSTERS; BORIDE;
D O I
10.3390/molecules29184304
中图分类号
Q5 [生物化学]; Q7 [分子生物学];
学科分类号
071010 ; 081704 ;
摘要
Water electrolysis has been recognized as a promising technology that can convert renewable energy into hydrogen for storage and utilization. The superior activity and low cost of catalysis are key factors in promoting the industrialization of water electrolysis. Single-atom catalysts (SACs) have attracted attention due to their ultra-high atomic utilization, clear structure, and highest hydrogen evolution reaction (HER) performance. In addition, the performance and stability of single-atom (SA) substrates are crucial, and various two-dimensional (2D) nanomaterial supports have become promising foundations for SA due to their unique exposed surfaces, diverse elemental compositions, and flexible electronic structures, to drive single atoms to reach performance limits. The SA supported by 2D nanomaterials exhibits various electronic interactions and synergistic effects, all of which need to be comprehensively summarized. This article aims to organize and discuss the progress of 2D nanomaterial single-atom supports in enhancing HER, including common and widely used synthesis methods, advanced characterization techniques, different types of 2D supports, and the correlation between structural hydrogen evolution performance. Finally, the latest understanding of 2D nanomaterial supports was proposed.
引用
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页数:44
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