Experimental investigation of styrene destruction in a non-thermal multi-arc plasma reactor with three pairs of electrodes

被引:0
作者
Zheng, Huan [1 ,2 ]
Ni, Guohua [1 ]
Sun, Hongmei [1 ]
Sui, Siyuan [1 ,2 ]
Ma, Zhongyang [1 ,2 ]
Zhao, Yanjun [3 ]
Li, Tiancheng [4 ]
Nie, Tingwei [4 ]
机构
[1] Chinese Acad Sci, Inst Plasma Phys, Hefei Inst Phys Sci, Hefei 230031, Peoples R China
[2] Univ Sci & Technol China, Sci Isl Branch, Grad Sch, Hefei, Peoples R China
[3] West Anhui Univ, Sch Mech & Vehicle Engn, Luan, Peoples R China
[4] Qingdao Donison Technol Co Ltd, Qingdao, Peoples R China
基金
中国国家自然科学基金;
关键词
Multi-arc; non-thermal plasma; styrene decomposition; thermal decomposition; degradation pathway; VOLATILE ORGANIC-COMPOUNDS; RELATIVE OSCILLATOR-STRENGTHS; DIELECTRIC BARRIER DISCHARGE; COMPOUNDS VOCS; CARBON-BLACK; TOLUENE; DECOMPOSITION; NAPHTHALENE; METHANE; REMOVAL;
D O I
10.1080/09593330.2025.2474258
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
A novel alternating current non-thermal multi-arc plasma generator with three pairs of electrodes was developed for styrene degradation. The experimental results indicated that multiple arcs enhance the destruction of styrene in the reactor. Styrene is not only thermally decomposed but also oxidatively degraded in the multi-arc reactor. When the concentration of styrene is not higher than 1200 mg/m(3), its removal rate can reach more than 90%. The major gaseous effluence products were CO and CO2. The solid product carbon black was found to be attached to the reactor wall. The main intermediates of styrene decomposition are butanol, ethyl acetate and benzaldehyde.
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页数:14
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共 56 条
  • [1] Plasma steam methane reforming (PSMR) using a microwave torch for commercial-scale distributed hydrogen production
    Akande, Olugbenga
    Lee, BongJu
    [J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2022, 47 (05) : 2874 - 2884
  • [2] Anicich VG., 2003, An index of the literature for bimolecular gas phase cation-molecule reaction kinetics
  • [3] Pilot scale degradation of mono and multi volatile organic compounds by surface discharge plasma/TiO2 reactor: Investigation of competition and synergism
    Assadi, Aymen Amine
    Loganathan, Sivachandiran
    Phuong Nguyen Tri
    Ghaida, Sara Gharib-Abou
    Bouzaza, Abdelkrim
    Anh Nguyen Tuan
    Wolbert, Dominique
    [J]. JOURNAL OF HAZARDOUS MATERIALS, 2018, 357 : 305 - 313
  • [4] Baba T, 2012, PRZ ELEKTROTECHNICZN, V88, P86
  • [5] BARD A, 1991, ASTRON ASTROPHYS, V248, P315
  • [6] Simulation of Naphthalene Conversion in Biogas Initiated by Pulsed Corona Discharges
    Bityurin, Valentin A.
    Filimonova, Elena A.
    Naidis, George V.
    [J]. IEEE TRANSACTIONS ON PLASMA SCIENCE, 2009, 37 (06) : 911 - 919
  • [7] PRECISION-MEASUREMENT OF RELATIVE OSCILLATOR-STRENGTHS .4. ATTAINMENT OF 0.5-PERCENT ACCURACY - FE-I TRANSITIONS FROM LEVELS A5 D0-4 (0.00-0.12 EV)
    BLACKWELL, DE
    IBBETSON, PA
    PETFORD, AD
    SHALLIS, MJ
    [J]. MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY, 1979, 186 (03) : 633 - 650
  • [8] MEASUREMENT OF RELATIVE OSCILLATOR-STRENGTHS FOR CR-I LINES .1. MEASURES FOR TRANSITIONS FROM LEVELS A7S3(0.00EV), A5S2(0.94EV) AND A5D0-4 (0.96-1.03EV)
    BLACKWELL, DE
    MENON, SLR
    PETFORD, AD
    [J]. MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY, 1984, 207 (03) : 533 - 546
  • [9] Plasma-enhanced chemical vapor deposition synthesis of vertically oriented graphene nanosheets
    Bo, Zheng
    Yang, Yong
    Chen, Junhong
    Yu, Kehan
    Yan, Jianhua
    Cen, Kefa
    [J]. NANOSCALE, 2013, 5 (12) : 5180 - 5204
  • [10] Carbon black processing by thermal plasma. Analysis of the particle formation mechanism
    Fabry, F
    Flamant, G
    Fulcheri, L
    [J]. CHEMICAL ENGINEERING SCIENCE, 2001, 56 (06) : 2123 - 2132