Simulation of selective catalytic reduction of NO and oxidation of CO and C7H8 over V2O5-TiO2 catalyst

被引:0
作者
Hua, Qingyuan [1 ]
Shen, Boxiong [1 ]
机构
[1] Hebei Univ Technol, Sch Energy & Environm Engn, Tianjin Key Lab Clean Energy & Pollut Control, Tianjin 300131, Peoples R China
基金
中国国家自然科学基金;
关键词
SCR; CO oxidation; Numerical simulation; Toluene oxidation; Monolithic honeycomb catalyst; NUMERICAL-SIMULATION; MANGANESE OXIDE;
D O I
10.1016/j.joei.2024.101956
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
A three-dimensional model of a single-channel honeycomb NH3-SCR catalytic converter was developed to simulate the catalytic reduction of NO and the simultaneous oxidation of CO and C7H8. The accuracy of the model was validated against experimental data. The effects of different operation conditions (such as space velocity, temperature, and inlet concentration) on the conversion efficiency of NO and CO were investigated, along with the distribution of gas components at various locations within the catalyst channel and along the catalyst wall. Compared to inlet gas concentrations, space velocity and temperature had a more significant impact on NO catalytic reduction and CO oxidation. Additionally, the oxidation behavior of toluene (C7H8) and its influence on the removal efficiency of NO and CO were analyzed by the simulation at the same time.
引用
收藏
页数:15
相关论文
共 53 条
  • [1] Study of the e+e- → π+ π- ω process at center-of-mass energies between 4.0 and 4.6 GeV
    Ablikim, M.
    Achasov, M. N.
    Adlarson, P.
    Albrecht, M.
    Aliberti, R.
    Amoroso, A.
    An, M. R.
    An, Q.
    Bai, Y.
    Bakina, O.
    Baldini Ferroli, R.
    Balossino, I.
    Ban, Y.
    Batozskaya, V.
    Becker, D.
    Begzsuren, K.
    Berger, N.
    Bertani, M.
    Bettoni, D.
    Bianchi, F.
    Bianco, E.
    Bloms, J.
    Bortone, A.
    Boyko, I.
    Briere, R. A.
    Brueggemann, A.
    Cai, H.
    Cai, X.
    Calcaterra, A.
    Cao, G. F.
    Cao, N.
    Cetin, S. A.
    Chang, J. F.
    Chang, W. L.
    Che, G. R.
    Chelkov, G.
    Chen, C.
    Chen, Chao
    Chen, G.
    Chen, H. S.
    Chen, M. L.
    Chen, S. J.
    Chen, S. M.
    Chen, T.
    Chen, X. R.
    Chen, X. T.
    Chen, Y. B.
    Chen, Z. J.
    Cheng, W. S.
    Choi, S. K.
    [J]. JOURNAL OF HIGH ENERGY PHYSICS, 2023, (08):
  • [2] Numerical analysis of NOx formation mechanisms and emission characteristics with different types of reactants dilution during MILD combustion of methane and coke oven gas
    Ali, Ghufran
    Zhou, Yuegui
    [J]. FUEL, 2022, 309
  • [3] The design and performance of GRD onboard the GECAM satellite
    An, Z. H.
    Sun, X. L.
    Zhang, D. L.
    Yang, S.
    Li, X. Q.
    Wen, X. Y.
    Gong, K.
    Liang, X. H.
    Liu, X. J.
    Liu, Y. Q.
    Li, Y. G.
    Xiong, S. L.
    Xu, Y. B.
    Zhang, Fan
    Zhao, X. Y.
    Cai, C.
    Chang, Z.
    Chen, G.
    Chen, C.
    Du, Y. Y.
    Feng, P. Y.
    Gao, M.
    Gao, R.
    Guo, D. Y.
    He, J. J.
    Hou, D. J.
    Li, C. Y.
    Li, G.
    Li, L.
    Li, X. F.
    Li, M. S.
    Lu, F. J.
    Lu, H.
    Meng, B.
    Peng, W. X.
    Shi, F.
    Wang, H.
    Wang, J. Z.
    Wang, Y. S.
    Wang, H. Z.
    Wen, X.
    Xiao, S.
    Xu, Y. P.
    Yang, J. W.
    Yi, Q. B.
    Zhang, S. N.
    Zhang, C. Y.
    Zhang, C. M.
    Zhang, Fei
    Zhao, Y.
    [J]. RADIATION DETECTION TECHNOLOGY AND METHODS, 2022, 6 (01) : 43 - 52
  • [4] THE BES DETECTOR
    BAI, JZ
    BIAN, Q
    CHEN, GM
    CHEN, LJ
    CHEN, SN
    CHEN, YQ
    CHEN, ZQ
    CHI, YK
    CUI, HC
    CUI, XZ
    DENG, SS
    DENG, YW
    DING, HL
    DONG, BZ
    DONG, XS
    DU, X
    DU, ZZ
    FENG, C
    FENG, Z
    FU, ZS
    GAO, CS
    GAO, ML
    GAO, SQ
    GAO, WX
    GAO, YN
    GU, SD
    GU, WX
    GUAN, YZ
    GUO, HF
    GUO, YN
    GUO, YY
    HAN, SW
    HAN, Y
    HAO, W
    HE, J
    HE, KR
    HE, MJ
    HOU, XJ
    HU, GY
    HU, JS
    HU, JW
    HUANG, DQ
    HUANG, YZ
    JIA, QP
    JIANG, CH
    JU, Q
    LAI, YF
    LANG, PF
    LI, DS
    LI, F
    [J]. NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT, 1994, 344 (02) : 319 - 334
  • [5] Influence of pretreatment conditions on low-temperature CO oxidation over Pd supported UiO-66 catalysts
    Bi, Fukun
    Zhang, Xiaodong
    Du, Quanxin
    Yue, Ke
    Wang, Ruizhuo
    Li, Fei
    Liu, Ning
    Huang, Yuandong
    [J]. MOLECULAR CATALYSIS, 2021, 509
  • [6] Bo Long-li, 2014, Huanjing Kexue, V35, P3302
  • [7] Catalytic performance over Mn-Ce catalysts for NH3-SCR of NO at low temperature: Different zeolite supports
    Chen, Lin
    Ren, Shan
    Liu, Lian
    Su, Buxin
    Yang, Jie
    Chen, Zhichao
    Wang, Mingming
    Liu, Qingcai
    [J]. JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING, 2022, 10 (02):
  • [8] TPD study of mordenite-type zeolites for selective catalytic reduction of NO by NH3
    Choi, EY
    Nam, IS
    Kim, YG
    [J]. JOURNAL OF CATALYSIS, 1996, 161 (02) : 597 - 604
  • [9] The catalytic activity of cobalt nanoparticles for low-temperature oxidation of carbon monoxide
    Dey, S.
    Dhal, G. C.
    [J]. MATERIALS TODAY CHEMISTRY, 2019, 14
  • [10] The universal character of the Mars and Van Krevelen mechanism
    Doornkamp, C
    Ponec, V
    [J]. JOURNAL OF MOLECULAR CATALYSIS A-CHEMICAL, 2000, 162 (1-2) : 19 - 32