Influence of Fuel and Technology on Particle Emissions from Biomass Cookstoves-Detailed Characterization of Physical and Chemical Properties

被引:0
作者
Lindgren, Robert [1 ]
Garcia-Lopez, Natxo [1 ]
Loven, Karin [2 ]
Lundin, Lisa [3 ]
Pagels, Joakim [2 ]
Boman, Christoffer [1 ]
机构
[1] Umea Univ, Dept Appl Phys & Elect, Thermochem Energy Convers Lab, SE-90187 Umea, Sweden
[2] Lund Univ, Ergon & Aerosol Technol, LTH, SE-22100 Lund, Sweden
[3] Umea Univ, Dept Chem, SE-90187 Umea, Sweden
来源
ACS OMEGA | 2025年 / 10卷 / 05期
基金
瑞典研究理事会;
关键词
SINGLE-PELLET COMBUSTION; TIME-RESOLVED ANALYSIS; PARTICULATE MATTER; FINE-PARTICLE; ASH TRANSFORMATION; GASEOUS EMISSIONS; HOUSEHOLD COOKING; WOOD COMBUSTION; AIR-POLLUTION; AEROSOL;
D O I
10.1021/acsomega.4c07785
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Globally, 3 billion people rely on solid biomass fuel for their everyday cooking, most often using inefficient cooking practices, leading to high exposure levels of household air pollution. This is subsequently associated with negative health and climate impact. Further, the inefficient use of biomass fuels applies pressure on natural forests, resulting in deforestation, loss of biodiversity, and soil degradation. Improved cookstove technologies and biomass fuels are being promoted to mitigate these issues. However, limited knowledge exists about how the interaction between stove technology and new fuels affects the physical and chemical properties of particulate emissions. In this study, the emission performance of four cookstove technologies in combination with five fuels was evaluated in a laboratory setup, applying a modified water boiling test with a hood dilution system for flue gas sampling. Filter sampling was applied to determine the emissions of fine particulate matter (PM1) and for subsequent analysis of polycyclic aromatic compounds (PAC), organic- and elemental carbon, and inorganic composition. Particle mass size distribution was determined by using a 13-stage low-pressure cascade impactor. Online instruments were used to determine gaseous emissions (e.g., CO, CH4, and BTX) as well as particle number size distribution. The results show that both the stove design and fuel properties influence the total emissions as well as the physiochemical PM characteristics. It was further seen that the impact of fuel on the PM properties did not translate linearly among the different stove technologies. This implies that each stove should be tested with various fuels to determine both the total emissions and fuel suitability.
引用
收藏
页码:4458 / 4472
页数:15
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