Integration of Pt3Ni Catalysts, Plasma-Etched Multiscale Membrane, and Flow Field with Micro-Channel for High-Performance Fuel Cell

被引:0
作者
Jang, Jue-Hyuk [1 ]
Seol, Changwook [2 ]
Jang, Segeun [3 ]
Lee, Jinwon [2 ]
Kim, Sang Moon [2 ]
Yoo, Sung Jong [1 ,4 ]
机构
[1] Korea Inst Sci & Technol, Hydrogen Fuel Cell Res Ctr, Seoul 02792, South Korea
[2] Incheon Natl Univ, Dept Mech Engn, Incheon 22012, South Korea
[3] Kookmin Univ, Sch Mech Engn, Seoul 02707, South Korea
[4] Univ Sci & Technol UST, KIST Sch, Div Energy & Environm Technol, Seoul 02792, South Korea
基金
新加坡国家研究基金会;
关键词
Fuel cell; Pt3Ni catalysts; Multiscale membrane; Plasma Etch; Flow Field with Micro-Channel; OXYGEN REDUCTION REACTION; FACILE PREPARATION; PEMFC; CARBON; NANOPARTICLES; SURFACE; INTERFACE; DESIGN;
D O I
10.1007/s40684-024-00690-0
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
To improve the performance and durability of polymer electrolyte membrane fuel cells, extensive research on each component has been performed, and there have been great advances for each part. However, no attempts have been made for the integration of all developed components into a PEMFC system. In this study, we successfully integrated a highly active Pt3Ni/C catalyst, a multiscale/multilevel membrane with a plasma etching process, and a flow-field bipolar plate with a micro-channel into a single-cell assembly, and achieved excellent PEMFC performance. Specifically, we obtained a maximum power density of more than 1.6 W/cm(2) with low catalyst loading of 0.125 mgPt/cm(2) (0.125 mgPtNi/cm(2)) at the anode (cathode) from the synergetic effects of the improved kinetics of oxygen reduction reaction, reduced ohmic resistance, and enhanced mass transport with the integration of each developed component. Furthermore, a current density of 2.61A/cm(2) at 0.6 V was achieved with catalyst loading of 0.2 mgPt/cm(2) (0.4 mgPtNi/cm(2)) at the anode (cathode).
引用
收藏
页数:9
相关论文
共 46 条
  • [1] Guided cracking of electrodes by stretching prism-patterned membrane electrode assemblies for high-performance fuel cells
    Ahn, Chi-Yeong
    Jang, Segeun
    Cho, Yong-Hun
    Choi, Jiwoo
    Kim, Sungjun
    Kim, Sang Moon
    Sung, Yung-Eun
    Choi, Mansoo
    [J]. SCIENTIFIC REPORTS, 2018, 8
  • [2] Numerical and experimental study of two-phase flow uniformity in channels of parallel PEM fuel cells with modified Z-type flow-fields
    Ashrafi, Moosa
    Kanani, Homayoon
    Shams, Mehrzad
    [J]. ENERGY, 2018, 147 : 317 - 328
  • [3] Bae JW, 2012, J IND ENG CHEM, V18, P876
  • [4] Facile preparation of carbon-supported PtNi hollow nanoparticles with high electrochemical performance
    Bae, Sung Jong
    Yoo, Sung Jong
    Lim, Yuntaek
    Kim, Sojeong
    Lim, Yirang
    Choi, Junghun
    Nahm, Kee Suk
    Hwang, Seung Jun
    Lim, Tae-Hoon
    Kim, Soo-Kil
    Kim, Pil
    [J]. JOURNAL OF MATERIALS CHEMISTRY, 2012, 22 (18) : 8820 - 8825
  • [5] Tailoring the Membrane-Electrode Interface in PEM Fuel Cells: A Review and Perspective on Novel Engineering Approaches
    Breitwieser, Matthias
    Klingele, Matthias
    Vierrath, Severin
    Zengerle, Roland
    Thiele, Simon
    [J]. ADVANCED ENERGY MATERIALS, 2018, 8 (04)
  • [6] Nanowire-in-Microtube Structured Core/Shell Fibers via Multifluidic Coaxial Electrospinning
    Chen, Hongyan
    Wang, Nu
    Di, Jiancheng
    Zhao, Yong
    Song, Yanlin
    Jiang, Lei
    [J]. LANGMUIR, 2010, 26 (13) : 11291 - 11296
  • [7] Multiplex lithography for multilevel multiscale architectures and its application to polymer electrolyte membrane fuel cell
    Cho, Hyesung
    Kim, Sang Moon
    Kang, Yun Sik
    Kim, Junsoo
    Jang, Segeun
    Kim, Minhyoung
    Park, Hyunchul
    Bang, Jung Won
    Seo, Soonmin
    Suh, Kahp-Yang
    Sung, Yung-Eun
    Choi, Mansoo
    [J]. NATURE COMMUNICATIONS, 2015, 6
  • [8] Just a Dream-or Future Reality?
    Gasteiger, Hubert A.
    Markovic, Nenad M.
    [J]. SCIENCE, 2009, 324 (5923) : 48 - 49
  • [9] Impact of land width and channel span on fuel cell performance
    Goebel, Steven G.
    [J]. JOURNAL OF POWER SOURCES, 2011, 196 (18) : 7550 - 7554
  • [10] One-Nanometer-Thick Pt3Ni Bimetallic Alloy Nanowires Advanced Oxygen Reduction Reaction: Integrating Multiple Advantages into One Catalyst
    Gong, Mingxing
    Deng, Zhiping
    Xiao, Dongdong
    Han, Lili
    Zhao, Tonghui
    Lu, Yun
    Shen, Tao
    Liu, Xupo
    Lin, Ruoqian
    Huang, Ting
    Zhou, Guangwen
    Xin, Huolin
    Wang, Deli
    [J]. ACS CATALYSIS, 2019, 9 (05) : 4488 - +