Insights into the morphology, composition, and sources of atmospheric particulate matter on Mount Qomolangma (Everest)

被引:1
作者
Tian, Biao [1 ]
Zhao, Peng [2 ,3 ,4 ]
Zhao, Pusheng [3 ,5 ]
Zhu, Kongju [1 ]
Tang, Jie [1 ,3 ]
Ding, Minghu [1 ]
机构
[1] Chinese Acad Meteorol Sci, Inst Global Change & Polar Res, Beijing 100081, Peoples R China
[2] Nankai Univ, Coll Environm Sci & Engn, State Environm Protect Key Lab Urban Ambient Air P, Tianjin 300350, Peoples R China
[3] Joint Lab Electron Microscopy Anal Atmospher Parti, Beijing 100012, Peoples R China
[4] NKU Cooperat Lab Atmospher Environm Hlth Res, CMA, Tianjin 300350, Peoples R China
[5] Beijing Met High Tech Co Ltd, Beijing 102200, Peoples R China
来源
JOURNAL OF ENVIRONMENTAL SCIENCES | 2025年 / 155卷
关键词
Mount Qomolangma; Particlulate matter; Single particle; Morphology analysis; Scanning electron microscope; MINERAL DUST PARTICLES; TIBETAN PLATEAU; SINGLE-SCATTERING; ICE NUCLEATION; BLACK CARBON; AEROSOL; SIZE; IRON; SIMULATIONS; DEPOSITION;
D O I
10.1016/j.jes.2024.06.006
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Aerosol category and its physicochemical properties are key factors influencing its climate and environmental effects. To further enhance our understanding of aerosols in the Himalayas-Tibetan Plateau region, atmospheric particulate matter samples were collected at three different altitudes on Mount Qomolangma (Everest). Using an automated scanning electron microscope system, the composition, size, and morphology of 52,349 particles were analyzed. The average mass concentrations of PM1, PM2.5, and PM10 were 0.678, 5.054, and 16.698 pg/m3, respectively. Aluminosilicate particles dominated the samples, accounting for 71.5% to 82.8% of PM10 mass and 34.7% to 62.4% of the particle number. Quartz particles, carbonate particles, metal oxides, and sulfates were also observed at different periods. Carbonaceous particles made up a significant portion of aerosols, comprising 2.1% to 9.7% of PM10 mass and 10.4% to 45.4% of particle number, with their concentration showing an upward trend with altitude. Small amounts of tar ball particles and fly ash particles were also observed, providing direct evidence of anthropogenic influences on high-altitude regions, even at altitudes exceeding 6000 m. The size distribution and abundance of different particle categories were closely related to the transport trajectories of air masses. The morphology of different particle categories varied, with fly ash particles mainly spherical and carbonaceous particles exhibiting higher irregularity. (c) 2025 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V.
引用
收藏
页码:889 / 900
页数:12
相关论文
共 66 条
[1]   The importance of feldspar for ice nucleation by mineral dust in mixed-phase clouds [J].
Atkinson, James D. ;
Murray, Benjamin J. ;
Woodhouse, Matthew T. ;
Whale, Thomas F. ;
Baustian, Kelly J. ;
Carslaw, Kenneth S. ;
Dobbie, Steven ;
O'Sullivan, Daniel ;
Malkin, Tamsin L. .
NATURE, 2013, 498 (7454) :355-358
[2]   Single-Particle SEM-EDX Analysis of Iron-Containing Coarse Particulate Matter in an Urban Environment: Sources and Distribution of Iron within Cleveland, Ohio [J].
Ault, Andrew P. ;
Peters, Thomas M. ;
Sawvel, Eric J. ;
Casuccio, Gary S. ;
Willis, Robert D. ;
Norris, Gary A. ;
Grassian, Vicki H. .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2012, 46 (08) :4331-4339
[3]   Global estimate of aerosol direct radiative forcing from satellite measurements [J].
Bellouin, N ;
Boucher, O ;
Haywood, J ;
Reddy, MS .
NATURE, 2005, 438 (7071) :1138-1141
[4]   Ice nucleating particles in the Saharan Air Layer [J].
Boose, Yvonne ;
Sierau, Berko ;
Isabel Garcia, M. ;
Rodriguez, Sergio ;
Alastuey, Andres ;
Linke, Claudia ;
Schnaiter, Martin ;
Kupiszewski, Piotr ;
Kanji, Zamin A. ;
Lohmann, Ulrike .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2016, 16 (14) :9067-9087
[5]   Elemental composition of aerosol in the Nam Co region, Tibetan Plateau, during summer monsoon season [J].
Cong, Zhiyuan ;
Kang, Shichang ;
Liu, Xiande ;
Wang, Guangfu .
ATMOSPHERIC ENVIRONMENT, 2007, 41 (06) :1180-1187
[6]   Elemental and individual particle analysis of atmospheric aerosols from high Himalayas [J].
Cong, Zhiyuan ;
Kang, Shichang ;
Dong, Shuping ;
Liu, Xiande ;
Qin, Dahe .
ENVIRONMENTAL MONITORING AND ASSESSMENT, 2010, 160 (1-4) :323-335
[7]   The Fifth International Workshop on Ice Nucleation phase 2 (FIN-02): laboratory intercomparison of ice nucleation measurements [J].
DeMott, Paul J. ;
Moehler, Ottmar ;
Cziczo, Daniel J. ;
Hiranuma, Naruki ;
Petters, Markus D. ;
Petters, Sarah S. ;
Belosi, Franco ;
Bingemer, Heinz G. ;
Brooks, Sarah D. ;
Budke, Carsten ;
Burkert-Kohn, Monika ;
Collier, Kristen N. ;
Danielczok, Anja ;
Eppers, Oliver ;
Felgitsch, Laura ;
Garimella, Sarvesh ;
Grothe, Hinrich ;
Herenz, Paul ;
Hill, Thomas C. J. ;
Hoehler, Kristina ;
Kanji, Zamin A. ;
Kiselev, Alexei ;
Koop, Thomas ;
Kristensen, Thomas B. ;
Krueger, Konstantin ;
Kulkarni, Gourihar ;
Levin, Ezra J. T. ;
Murray, Benjamin J. ;
Nicosia, Alessia ;
O'Sullivan, Daniel ;
Peckhaus, Andreas ;
Polen, Michael J. ;
Price, Hannah C. ;
Reicher, Naama ;
Rothenberg, Daniel A. ;
Rudich, Yinon ;
Santachiara, Gianni ;
Schiebel, Thea ;
Schrod, Jann ;
Seifried, Teresa M. ;
Stratmann, Frank ;
Sullivan, Ryan C. ;
Suski, Kaitlyn J. ;
Szakall, Miklos ;
Taylor, Hans P. ;
Ullrich, Romy ;
Vergara-Temprado, Jesus ;
Wagner, Robert ;
Whale, Thomas F. ;
Weber, Daniel .
ATMOSPHERIC MEASUREMENT TECHNIQUES, 2018, 11 (11) :6231-6257
[8]   Complex refractive indices and single-scattering albedo of global dust aerosols in the shortwave spectrum and relationship to size and iron content [J].
Di Biagio, Claudia ;
Formenti, Paola ;
Balkanski, Yves ;
Caponi, Lorenzo ;
Cazaunau, Mathieu ;
Pangui, Edouard ;
Journet, Emilie ;
Nowak, Sophie ;
Andreae, Meinrat O. ;
Kandler, Konrad ;
Saeed, Thuraya ;
Piketh, Stuart ;
Seibert, David ;
Williams, Earle ;
Doussin, Jean-Francois .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2019, 19 (24) :15503-15531
[9]   Present-day climate forcing and response from black carbon in snow [J].
Flanner, Mark G. ;
Zender, Charles S. ;
Randerson, James T. ;
Rasch, Philip J. .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2007, 112 (D11)
[10]   Recent progress in understanding physical and chemical properties of African and Asian mineral dust [J].
Formenti, P. ;
Schuetz, L. ;
Balkanski, Y. ;
Desboeufs, K. ;
Ebert, M. ;
Kandler, K. ;
Petzold, A. ;
Scheuvens, D. ;
Weinbruch, S. ;
Zhang, D. .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2011, 11 (16) :8231-8256