The role of excitations in supercooled liquids: Density, geometry, and relaxation dynamics

被引:0
|
作者
Ji, Wencheng [1 ]
Ciamarra, Massimo Pica [2 ,3 ]
Wyart, Matthieu [4 ]
机构
[1] Weizmann Inst Sci, Dept Phys Complex Syst, IL-76100 Rehovot, Israel
[2] Nanyang Technol Univ, Div Phys & Appl Phys, Sch Phys & Math Sci, Singapore 637371, Singapore
[3] CNR, CNR SPIN, I-80126 Naples, Italy
[4] Ecole Polytech Fed Lausanne, Inst Phys, CH-1015 Lausanne, Switzerland
基金
瑞士国家科学基金会;
关键词
glass; excitation; landscape; GLASS-TRANSITION; BREAKDOWN;
D O I
10.1073/pnas.2416800122
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Low-energy excitations play a key role in all condensed-matter systems, yet there is limited understanding of their nature in glasses, where they correspond to local rearrangements of groups of particles. Here, we introduce an algorithm to systematically uncover these excitations up to the activation energy scale relevant to structural relaxation. We use it in a model system to measure the density of states on a scale never achieved before, confirming that this quantity shifts to higher energy under cooling, precisely as the activation energy does. Second, we show that the excitations' energetic and spatial features allow one to predict with great accuracy the dynamic propensity, i.e., the location of future relaxation dynamics. Finally, we find that excitations have a primary field whose properties, including the displacement of the most mobile particle, scale as a power-law of their activation energy and are independent of temperature. Additionally, they exhibit an outer deformation field that depends on the material's stability and, therefore, on temperature. We build a scaling description of these findings. Overall, our analysis supports that excitations play a crucial role in regulating relaxation dynamics near the glass transition, effectively suppressing the transition to dynamical arrest predicted by mean-field theories while also being strongly influenced by it.
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页数:8
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