Use of clay honeycomb monoliths for the removal of tetracycline antibiotic from water

被引:0
|
作者
Sumariva, Felix [1 ,2 ,3 ,4 ]
Moreno-Dorado, F. Javier [3 ,4 ]
Guerra, Francisco M. [3 ,4 ]
Goma, Daniel [1 ,2 ,5 ]
Vidal, Hilario [1 ,2 ]
Gatica, Jose Manuel [1 ,2 ]
机构
[1] Univ Cadiz, Dept Ciencia Mat Ingn Met & Quim Inorgan, Puerto Real 11510, Spain
[2] Univ Cadiz, Inst Microscopia Elect & Mat IMEYMAT, Puerto Real 11510, Spain
[3] Univ Cadiz, Dept Quim Organ, Puerto Real 11510, Spain
[4] Univ Cadiz, Inst Biomol INBIO, Puerto Real 11510, Spain
[5] Queens Univ Belfast, Sch Chem & Chem Engn, David Keir Bldg,Strandmillis Rd, Belfast BT9 5AG, North Ireland
关键词
Adsorption; Clay; Honeycomb monolith; Tetracycline; Water; Antibiotics; OIL PALM ASH; METHYLENE-BLUE; DEGRADATION-PRODUCTS; NATURAL CLAYS; COMPOSITE; ADSORPTION; ADSORBENT; TOXICITY;
D O I
10.1016/j.jwpe.2024.106381
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
This study assesses the efficacy of natural clays as a cost-effective and ecologically sound method for the removal of tetracycline from water. A notable advancement in the field of antibiotic removal is the utilization of honeycomb monoliths in lieu of traditional powder-based materials. The objective of this approach is to facilitate easier handling and to mitigate the production of sludge. The findings illustrate that, among the five clay types studied, the kerolitic montmorillonite is particularly effective in removing tetracycline from water, achieving levels of approximately 100 mg/g. This effectiveness is remarkably consistent across a range of pH levels (both acidic and basic), temperatures (4-60 degrees C), and even flow rates when employing the honeycomb design (50-2800 mL/min). These results substantiate the efficacy of this approach as a robust and promising strategy for wastewater treatment. In light of the fact that the principal mechanism of action for these clays is adsorption, the study also addresses ancillary concerns such as filter cleaning for reuse and the complete elimination of tetracycline.
引用
收藏
页数:10
相关论文
共 50 条
  • [1] Clay honeycomb monoliths for the simultaneous retention of lead and cadmium in water
    Ahrouch, Mohammadi
    Gatica, Jose Manuel
    Draoui, Khalid
    Bellido-Milla, Dolores
    Vidal, Hilario
    ENVIRONMENTAL TECHNOLOGY & INNOVATION, 2022, 27
  • [2] Study of the nickel removal from water applying Design of Experiments and using natural clay honeycomb monoliths
    Bellido-Milla, Dolores
    Vidal, Hilario
    Nunez, Maria
    Ahrouch, Mohammadi
    Gatica, Jose M.
    JOURNAL OF WATER PROCESS ENGINEERING, 2023, 55
  • [3] TETRACYCLINE REMOVAL FROM WATER BY ADSORPTION ON GEOMATERIAL, ACTIVATED CARBON AND CLAY ADSORBENTS
    Ait Hamoudi, Souhila
    Hamdi, Boualem
    Brendle, Jocelyne
    ECOLOGICAL CHEMISTRY AND ENGINEERING S-CHEMIA I INZYNIERIA EKOLOGICZNA S, 2021, 28 (03): : 303 - 328
  • [4] Clay-biochar composites for sorptive removal of tetracycline antibiotic in aqueous media
    Premarathna, K. S. D.
    Rajapaksha, Anushka Upamali
    Adassoriya, Nadeesh
    Sarkar, Binoy
    Sirimuthu, Narayana M. S.
    Cooray, Asitha
    Ok, Yong Sik
    Vithanage, Meththika
    JOURNAL OF ENVIRONMENTAL MANAGEMENT, 2019, 238 : 315 - 322
  • [5] Clay and Zeolite-Clay Based Monoliths as Adsorbents for the Hg(II) Removal from the Aqueous Solutions
    Darmadi
    Lubis, Mirna Rahmah
    Masrura, Munadiya
    Syahfatra, Aziz
    Mahidin
    INTERNATIONAL JOURNAL OF TECHNOLOGY, 2023, 14 (01) : 129 - 141
  • [6] Comprehensive evaluation of antibiotic tetracycline and oxytetracycline removal by Fe-metal organic framework/biopolymer-clay hydrogel
    Cha, Byungjun
    Kim, Nahyun
    Yea, Yeonji
    Han, Jonghun
    Yoon, Yeomin
    Kim, Sewoon
    Park, Chang Min
    CERAMICS INTERNATIONAL, 2023, 49 (08) : 12201 - 12213
  • [7] Synthesis of hydroxyapatite/clay and hydroxyapatite/pumice composites for tetracycline removal from aqueous solutions
    Ersan, Mehtap
    Guler, Ulker Asli
    Acikel, Unsal
    Sarioglu, Meltem
    PROCESS SAFETY AND ENVIRONMENTAL PROTECTION, 2015, 96 : 22 - 32
  • [8] Sorptive removal of tetracycline from water by palygorskite
    Chang, Po-Hsiang
    Li, Zhaohui
    Yu, Tsai-Luen
    Munkhbayer, Sandagdori
    Kuo, Tzu-Hsing
    Hung, Yu-Chiao
    Jean, Jiin-Shuh
    Lin, Kao-Hung
    JOURNAL OF HAZARDOUS MATERIALS, 2009, 165 (1-3) : 148 - 155
  • [9] Mechanistic insight into efficient removal of tetracycline from water by Fe/graphene
    Alatalo, Sara-Maaria
    Daneshvar, Ehsan
    Kinnunen, Niko
    Mesceriakovas, Arunas
    Thangaraj, Senthil K.
    Janis, Janne
    Tsang, Daniel C. W.
    Bhatnagar, Amit
    Lahde, Anna
    CHEMICAL ENGINEERING JOURNAL, 2019, 373 : 821 - 830
  • [10] Easy route to activate clay honeycomb monoliths for environmental applications
    Cifredo, Gustavo
    Manuel Gatica, Jose
    Harti, Sanae
    Vidal, Hilario
    APPLIED CLAY SCIENCE, 2010, 47 (3-4) : 392 - 399