To address the urgent demand for autonomous rapid initial alignment of vehicular inertial navigation systems in complex battlefield environments, this study overcomes the technical limitations of traditional stationary base alignment methods by proposing a robust moving-base autonomous alignment approach based on multi-source information fusion. First, a federal Kalman filter-based multi-sensor fusion architecture is established to effectively integrate odometer, laser Doppler velocimeter, and SINS data, resolving the challenge of autonomous navigation parameter calculation under GNSS-denied conditions. Second, a dual-mode fault diagnosis and isolation mechanism is developed to enable rapid identification of sensor failures and system reconfiguration. Finally, an environmentally adaptive dynamic alignment strategy is proposed, which intelligently selects optimal alignment modes by real-time evaluation of motion characteristics and environmental disturbances, significantly enhancing system adaptability in complex operational scenarios. The experimental results show that the method proposed in this paper can effectively improve the accuracy of vehicle-mounted alignment in motion, achieve accurate identification, effective isolation, and reconstruction of random incidental faults, and improve the adaptability and robustness of the system. This research provides an innovative solution for the rapid deployment of special-purpose vehicles in GNSS-denied environments, while its fault-tolerant mechanisms and adaptive strategies offer critical insights for engineering applications of next-generation intelligent navigation systems.