Microporous carbon derived from waste plastics for efficient adsorption of tetracycline: Adsorption mechanism and application potentials

被引：0

作者：

Bian, Shiyu ^{[1
]}

Cai, Zhuoyu ^{[1
]}

Xing, Weinan ^{[1
]}

Zhao, Chunyu ^{[3
]}

Pan, Yuwei ^{[1
]}

Han, Jiangang ^{[4
]}

Wu, Guangyu ^{[1
,2
]}

Huang, Yudong ^{[5
]}

机构：

[1] Nanjing Forestry Univ, Coll Ecol & Environm, Coinnovat Ctr Sustainable Forestry Southern China, Nanjing 210037, Peoples R China

[2] Guangxi Univ, Guangxi Key Lab Petrochem, Resource Proc & Proc Intensificat Technol, Sch Chem & Chem Engn, Nanning 530004, Peoples R China

[3] Shandong First Med Univ & Shandong Acad Med Sci, Sch Chem & Pharmaceut Engn, Tai An 271016, Peoples R China

[4] Changzhou Inst Technol, Sch Chem Engn & Mat, Changzhou 213032, Peoples R China

[5] Harbin Inst Technol, Sch Chem & Chem Engn, MIIT Key Lab Crit Mat Technol New Energy Convers &, Harbin 150001, Peoples R China

来源：

ENVIRONMENTAL RESEARCH | 2025年 / 268卷

关键词：

Waste plastic utilization; Adsorbent; Tetracycline removal; ACTIVATED CARBONS; ANTIBIOTICS; REMOVAL;

D O I：

10.1016/j.envres.2025.120785

中图分类号：

X [环境科学、安全科学];

学科分类号：

08 ; 0830 ;

摘要：

In recent years, the accumulation of waste plastics and emergence plastic-derived pollutants such as microplastics have driven significantly the development and updating of waste plastic utilization technology. This study prepared the porous carbon (PC-1-KOH) material directly from polyethylene terephthalate (PET) in waste plastic bottles using KOH activation and molten salt strategy for efficient removal of antibiotic tetracycline (TC). The maximum removal efficiency of TC was 100.0% with a PC-1-KOH weight of 20 mg. In addition, the TC removal efficiency stayed over 80.0% within the rage of pH of 3-9 and different water bodies. The adsorption process was described by the Pseudo-second-order kinetic model and the Langmuir isotherm, suggesting that the adsorption of TC was predominantly chemical in nature and occurred on a homogeneous surface. The pores filling, hydrogen bonding, it-it stacking interactions and electrostatic interaction are the main mechanisms of TC adsorption. This work demonstrates a sustainable approach to converting plastic waste derived materials into functional materials for effective pollution removal and environmental remediation.

引用

页数：10

共 71 条

[71]

Zheng X., Et al., Enhanced degradation of ciprofloxacin by graphitized mesoporous carbon (GMC)-TiO<sub>2</sub> nanocomposite: strong synergy of adsorption-photocatalysis and antibiotics degradation mechanism, J. Colloid Interface Sci., 527, pp. 202-213, (2018)

← 1 2 3 4 5 6 7 8 →