One-Dimensional Plasmons and Hybridized Coupled Polaritons in Carbon Nanotubes

被引:0
作者
Kestyn, James [1 ]
Yngvesson, Sigfrid K. [1 ]
Polizzi, Eric [1 ]
机构
[1] Univ Massachusetts, Dept Elect & Comp Engn, Amherst, MA 01003 USA
基金
美国国家科学基金会;
关键词
SINGLE-MOLECULE; RESONANCES; GRAPHENE; MODEL; TIME;
D O I
10.1021/acs.jpcc.4c07547
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
This paper presents real-time time-dependent density functional theory (TDDFT) ab initio simulations of selected armchair carbon nanotubes (CNTs). By scaling the lengths of CNTs, we provide a comprehensive analysis of the Tomonaga-Luttinger (T-L) 1-D plasmon velocities, confirming consistency with theoretical predictions and experimental observations. Our findings include detailed visual representations of excitation densities at various resonances. Furthermore, we explore the coupling between T-L plasmons and single electron excitations, identifying distinct 1-D polariton behaviors, such as strong harmonic generation due to nonlinearities, as well as energy gaps that differ from conventional 2-D polaritons. The study highlights the unique properties of armchair single-walled carbon nanotubes as low-loss nanocavity resonators, demonstrating potential applications in strong light-matter coupling and other nanophotonic devices. The simulation framework employed here opens avenues for further research into 1-D plasmonic phenomena and electronic spectroscopy in complex nanostructures.
引用
收藏
页码:2062 / 2073
页数:12
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